Journal
CHEMISTRY OF MATERIALS
Volume 27, Issue 4, Pages 1233-1241Publisher
AMER CHEMICAL SOC
DOI: 10.1021/cm504033r
Keywords
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Funding
- JSPS KAKENHI [25420724]
- MEXT Program for Development of Environmental Technology using Nanotechnology
- World Premier International Research Center (WPI) Initiative on Materials Nanoarchitectonics, a program of the Ministry of Education, Culture, Sports, Science and Technology, Japan (MEXT)
- Grants-in-Aid for Scientific Research [25420724] Funding Source: KAKEN
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This paper reports on the epitaxial growth of Li3xLa2/3-xTiO3 thin films by means of pulsed laser deposition and their transport properties. A series of films obtained in this study have revealed that the thin film quality and Li-ion conductivity are highly sensitive to growth conditions as well as target composition. The epitaxial thin films are mostly c-axis oriented, containing a small amount of a-axis domains and antiphase boundaries. In-plane conductivity measurements investigating the relationship between these defects and Li-ion conductivity in Li3xLa2/3-xTiO3 show that the defects are not predominantly resistive against the ionic conduction.
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