Journal
CHEMISTRY OF MATERIALS
Volume 27, Issue 4, Pages 1405-1411Publisher
AMER CHEMICAL SOC
DOI: 10.1021/cm5047269
Keywords
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Funding
- National Natural Science Foundation of China [21373097, 51072067]
- National Basic Research Program of China [2011CB935800]
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Single-phase greener phosphor with broadband emission made of colloidal quantum dots (QDs) is most desirable for use as color convertors in white light-emitting diodes (WLEDs). Here, we demonstrate a single cadmium-free component system consisting of Cu-doped InP core/ZnS barrier/InP quantum well/ZnS shell QDs, which exhibits two emission peaks by controlling the barrier thickness under single-excitation wavelength, one of which being attributed to Cu-doped InP, and the other resulting from InP quantum well. The dual emissive peaks were successfully tuned in a range from visible to near-infrared by simple control of the core size and the well thickness, respectively. Using optimal structures as color converters, we successfully obtained WLED with a color rending index (CRI) up to 91 and CIE color coordinates of (0.338, 0.330) by combination with blue LED chip, indicating this single-phase phosphor with great promise for use in solid-state lighting due to flexibly tunable dual emission peak position in the entire visible region.
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