Journal
NEW JOURNAL OF CHEMISTRY
Volume 40, Issue 7, Pages 6001-6004Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6nj01076h
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TaOx grafted onto Al2O3 is investigated for C-N bond cleavage of amines under H-2 pressure. Heteroaromatics such as aniline are stoichiometrically denitrogenated at high temperature, while cyclohexylamine is catalytically denitrogenated. UV-visible and X-ray photoelectron spectroscopy indicate the formation of a stable Ta-N species in the former case.
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