Journal
CHEMICAL SOCIETY REVIEWS
Volume 44, Issue 17, Pages 6018-6034Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c5cs00198f
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Funding
- National Natural Science Foundation of China [21422306, 21333009, 21273197]
- National High-Tech Research and Development program of China [2013AA065301]
- Fundamental Research Funds for the Central Universities [2015XZZX004-04]
- Zhejiang Provincial Natural Science Foundation of China [LR15B030001]
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The emergence of porous organic polymers (POPs) has provided great opportunities for new applications in heterogeneous catalysis owing to their unprecedented intrinsic structural features such as high surface areas, extraordinary framework stabilities and chemically adjustable compositions. In this tutorial review, representative recent developments in the POPs-based catalysts with hierarchically porous structures are presented. Various strategies for the syntheses of hierarchically porous polymers including hard-templating, soft-templating and template-free approaches and the design of catalytically active porous polymers including post-modification, co-polymerization and self-polymerization have been discussed. In addition, their catalytic properties are compared. Finally, we emphasize the importance of the synthesis of hierarchically porous polymer based heterogeneous catalysts using sustainable routes under template-free and metal-free conditions.
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