Journal
CHEMICAL RECORD
Volume 15, Issue 4, Pages 728-742Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/tcr.201500005
Keywords
asymmetric synthesis; electrophilic cyclization; lactonization; Lewis bases; organocatalysis
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Funding
- MEXT KAKENHI [26105739]
- Grants-in-Aid for Scientific Research [26105739, 15H05810, 15H05755] Funding Source: KAKEN
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Electrophilic cyclizations of unactivated alkenes play highly important roles in the synthesis of useful building blocks. This account describes our contributions to the rational design of monofunctionalized chiral Lewis base catalysts for enantioselective iodo- and protocyclizations. For the stereoselective promotion of electrophilic bromocyclizations, nucleophilic phosphite-urea cooperative catalysts have been designed.
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