4.8 Article

Magnetic-field-enhanced high thermoelectric performance in narrow-band-gap polycrystalline semiconductor Ag2+8Te

Journal

MATERIALS TODAY PHYSICS
Volume 36, Issue -, Pages -

Publisher

ELSEVIER
DOI: 10.1016/j.mtphys.2023.101161

Keywords

Ag2Te; Magneto-thermoelectric effects; Thermoelectrics; Narrow-band-gap semiconductors

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The thermoelectric performance of polycrystalline Ag2+8Te can be enhanced by a magnetic field, increasing its ZT value from 0.44 to 0.80 at 300 K. This suggests that external field regulation can be an effective strategy to improve thermoelectric properties.
Ag2Te is a promising near-room-temperature thermoelectric material. However, its thermoelectric performance is difficult to be further improved by traditional strategies, such as doping and alloying. Herein, we demonstrate that the magnetic field is effective to enhance the thermoelectric performance of polycrystalline Ag2+8Te. The ZT of Ag2+8Te at 300 K can increase from 0.44 to 0.80 under a perpendicular magnetic field of 5 T. Similar to the magneto-thermoelectric properties observed in the semimetal materials, our studies not only reveal that the linear energy dispersion plays an important role for the increase of ZT in polycrystalline Ag2+8Te, but also suggest that external field regulation can be an effective strategy to enhance the thermoelectric properties.

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