Magneto-optical effects in lead halide perovskites

Lead halide perovskites have emerged as promising semiconductors for high-performance photovoltaics, light-emitting devices as well as quantum information technologies. In this review, we highlight the magneto-optical effects in these materials from both fundamental research and practical application perspectives. We summarize the experimental results measured for basic physical quantities and the assignment of various spectral peaks using the magneto-optical spectroscopy. These results provide a solid foundation underlying the excellent photo-electronic properties of lead halide perovskites. Additionally, we provide an overview of carrier spin precession and its hyperfine interaction with the nuclear spin bath in response to the applied magnetic field, which is essential for developing perovskite-based spintronic devices. We also illustrate the magnetic-field effects in optoelectronic devices, aiming at providing instructions for performance optimization. Finally, we discuss several challenging research directions towards a comprehensive understanding of the perovskite family and their potential applications in quantum physics, which might be accessed with the magneto-optical techniques. Overall, this review highlights the intriguing possibilities for lead halide perovskites in magneto-optical research and technology, and provides insights for future investigations to advance this promising field.

Automated summary

This review focuses on the magneto-optical effects in lead halide perovskites and summarizes the experimental results and interpretations of various spectral peaks. The response of carrier spin precession and its interaction with the nuclear spin bath to an applied magnetic field is outlined, along with the magnetic-field effects in optoelectronic devices. The potential applications of perovskite family in quantum physics are discussed, and future research directions are proposed.