Journal
NANOSCALE
Volume 8, Issue 3, Pages 1652-1657Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c5nr07345f
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Funding
- National Basic Research Program of China [2011CB932303, 2013CB934203, 2012CB933001]
- Chinese Academy of Sciences [YZ201318]
- National Natural Science Foundation of China [21472029, 51173031, 91127043, 21372136]
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The self-assembly of a tetrathiafulvalene (TTF) derivative (EDTTF) and a 1,3,5-tris(10-carboxydecyloxy)-benzene (TCDB) heterobilayer nanostructure at the 1-phenyloctane/HOPG interface under ambient conditions has been studied by scanning tunneling microscopy (STM). EDTTF and TCDB could co-assemble into a brand new hexagonal network with one of the largest nano-cavities. Finally, the nanoporous network would transform into a more stable linear structure. Density functional theory (DFT) calculations have been performed to reveal the formation mechanism.
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