Carbon-Doped Co2MnSi Heusler Alloy Microwires with Improved Thermal Characteristics of Magnetization for Multifunctional Applications

In the current work, we illustrate the effect of adding a small amount of carbon to very common Co2MnSi Heusler alloy-based glass-coated microwires. A significant change in the magnetic and structure structural properties was observed for the new alloy Co2MnSiC compared to the Co2MnSi alloy. Magneto-structural investigations were performed to clarify the main physical parameters, i.e., structural and magnetic parameters, at a wide range of measuring temperatures. The XRD analysis illustrated the well-defined crystalline structure with average grain size (D-g = 29.16 nm) and a uniform cubic structure with A2 type compared to the mixed L2(1) and B2 cubic structures for Co2MnSi-based glass-coated microwires. The magnetic behavior was investigated at a temperature range of 5 to 300 K and under an applied external magnetic field (50 Oe to 20 kOe). The thermomagnetic behavior of Co2MnSiC glass-coated microwires shows a perfectly stable behavior for a temperature range from 300 K to 5 K. By studying the field cooling (FC) and field heating (FH) magnetization curves at a wide range of applied external magnetic fields, we detected a critical magnetic field (H = 1 kOe) where FC and FH curves have a stable magnetic behavior for the Co2MnSiC sample; such stability was not found in the Co2MnSi sample. We proposed a phenomenal expression to estimate the magnetization thermal stability, & UDelta;M (%), of FC and FH magnetization curves, and the maximum value was detected at the critical magnetic field where & UDelta;M (%) & AP; 98%. The promising magnetic stability of Co2MnSiC glass-coated microwires with temperature is due to the changing of the microstructure induced by the addition of carbon, as the A2-type structure shows a unique stability in response to variation in the temperature and the external magnetic field. In addition, a unique internal mechanical stress was induced during the fabrication process and played a role in controlling magnetic behavior with the temperature and external magnetic field. The obtained results make Co2MnSiC a promising candidate for magnetic sensing devices based on Heusler glass-coated microwires.

Automated summary

This study investigates the effect of adding a small amount of carbon to Co2MnSi Heusler alloy-based glass-coated microwires. The newly developed Co2MnSiC alloy shows significant changes in magnetic and structural properties compared to the Co2MnSi alloy. The results suggest that Co2MnSiC has promising magnetic stability and is a potential candidate for magnetic sensing devices.