Journal
NATURE COMMUNICATIONS
Volume 14, Issue 1, Pages -Publisher
NATURE PORTFOLIO
DOI: 10.1038/s41467-023-42459-0
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The study discovered a new fermionic quadrupling condensate that breaks the Z(2) time-reversal symmetry. By detecting the specific heat, researchers found specific anomalies above the superconducting critical temperature, which are associated with the broken time-reversal symmetry.
Materials that break multiple symmetries allow the formation of four-fermion condensates above the superconducting critical temperature (T-c). Such states can be stabilized by phase fluctuations. Recently, a fermionic quadrupling condensate that breaks the Z(2) time-reversal symmetry was reported in Ba1-xKxFe2As2. A phase transition to the new state of matter should be accompanied by a specific heat anomaly at the critical temperature where Z(2) time-reversal symmetry is broken (T-c(Z2)>T-c). Here, we report on detecting two anomalies in the specific heat of Ba1-xKxFe2As2 at zero magnetic field. The anomaly at the higher temperature is accompanied by the appearance of a spontaneous Nernst effect, indicating the breakdown of Z(2) symmetry. The second anomaly at the lower temperature coincides with the transition to a zero-resistance state, indicating the onset of superconductivity. Our data provide the first example of the appearance of a specific heat anomaly above the superconducting phase transition associated with the broken time-reversal symmetry due to the formation of the novel fermion order.
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