Journal
LANGMUIR
Volume 39, Issue 36, Pages 12826-12834Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.langmuir.3c01689
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A recent study has revealed the nontrivial dynamics of liquid drops impacting on soft surfaces, particularly during the later stages before settling. The relative viscosity of the liquid drop, the liquid layer, and the intrinsic wettability of the solid substrate play significant roles in governing the post-collision dynamics. Surprisingly, the viscous liquid layer can reduce viscous dissipation and accelerate the drop's final settlement.
A liquid drop impacting on a soft surface is known to exhibit fascinating dynamics that is distinctive from its bounce-back atop a rigid surface. However, while the early spreading of the drop subsequent to its immediate impact with a lubricating liquid layer appears to be reasonably well understood, the later events of retraction and eventual stabilization appear to be poorly addressed. Here, we bring out the nontrivial confluence of the solid substrate wettability and the liquid layer viscosity toward modulating the post-collision dynamics of an impinging liquid drop on a viscous oil-infused surface during its later phase of settlement before arriving at an equilibrium state. Our results reveal that despite an intuitive analogy with the classical phenomenon of damped oscillation, the drop, during its later stages of motion, undergoes dynamical events that may be nontrivially dictated by not only the relative viscosity of the impacting drop and the liquid layer but also the intrinsic wettability of the solid substrate, governing its post-impact settlement via a sequel of spreading-retraction cycles. As a consequence, the viscous liquid layer, instead of providing additional damping, may nonintuitively reduce the effective viscous dissipation so as to hasten the drop's final settlement. These results may turn out to be critical in designing engineered surfaces for tuning the movement of drops in a preferential pathway, bearing decisive implications in the functionalities of liquid lenses, inkjet printing, spray coating and cooling, and several other emerging applications in the realm of lubricated fluidic interfaces.
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