Journal
JOURNAL OF POWER SOURCES
Volume 580, Issue -, Pages -Publisher
ELSEVIER
DOI: 10.1016/j.jpowsour.2023.233456
Keywords
Microfluidic; Membraneless; Microfabricated; Self-pumping; Disposable; Hybrid biofuel cell
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This paper presents a novel design and operation of microbial fuel cells (\MFCs) with monolayer paper-based substrate/electrodes and microchannels with co-laminar flow. The performance is significantly improved with the incorporation of a double-inlet and diverging channel design. The developed MFCs achieve a peak power density of 19.4μW cm-2 and maximum current density of 190.4μA cm-2, surpassing the performance of previously reported paper-based single MFCs.
This paper presents a novel design and operation of microbial fuel cells (\MFCs), which contain monolayer paper -based substrate/electrodes and microchannels with co-laminar flow. The electrodes with multi-wall carbon nanotubes are fabricated by the screen-printing method and the microchannels are patterned using photo-lithography. A double-inlet and diverging channel design is incorporated in the fuel cell configuration and demonstrated significantly improved performance. The fluid flows of electrolytes through the porous paper media are simulated using steady-state and transient computational fluid dynamics The best performance is achieved under the following conditions: an electroactive microbial (S. oneidensis) concentration of OD6001.5, 50 mM electron donor (lactate), and direct immobilized of the inoculum on the anode surface. The developed MFCs achieves a peak power density of 19.4 & PLUSMN; 0.23 & mu;W cm-2 and maximum current density of 190.4 & PLUSMN; 1.39 & mu;A cm-2, surpassing the performance of all previously reported paper-based single MFCs that utilize paper-based elec-trodes. In addition, hybrid-type MFCs that containing enzymatic air-breathing cathodes are investigated to enhance their performance. The novel paper based self-pumping MFC has the potential to make lab-on-a-chip type portable medical diagnosis devices with integrated power sources practical and feasible.
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