4.8 Article

Enhanced Rashba Spin Orbit Coupling and Magnetic Behavior at Oxide Heterointerfaces by Optical Gating

Journal

JOURNAL OF PHYSICAL CHEMISTRY LETTERS
Volume 14, Issue 38, Pages 8684-8690

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acs.jpclett.3c01811

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Complex oxide heterointerfaces have rich physical phenomena and broad quantum coherence, and light can be used to manipulate properties and observe interesting physical phenomena, such as enhanced magnetoresistance.
Complex oxide heterointerfaces have been a hot research spot due to their rich physical phenomena and broad quantum coherence that respond to multiple external stimuli. Among these external stimuli, light is a very powerful one to manipulate properties such as carrier density and spin characteristics. However, achieving a light-magnetic correlation is in high demand for multifield responding devices, and its intrinsic mechanism remains unclear. Here, by illuminating Nd0.86Sr0.14Al0.86Ni0.14O3-SrTiO3 heterointerfaces using 360 nm light, we observe a series of interesting physical phenomena, like enhanced magnetoresistance (MR). More interestingly, a band splitting and strong Rashba spin-orbit coupling (SOC) effect occur after illumination, accompanied by a magnetic feature and thus leading to an anomalous Hall effect (AHE). Upon optical gating, the magnetism can be caused by Rashba SOC induced spin-orbit torque (SOT). The work will be sure to have great importance in both theoretical studies and all-oxide devices.

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