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MengBi Zhang et al.
Summary: In this paper, a Mo-doped Nickel-iron selenide catalyst grown on nickel foam was synthesized by two hydrothermal reactions and exhibited excellent catalytic performance for both hydrogen evolution reactions (HER) and oxygen evolution reactions (OER) in 1 mol/L KOH electrolyte. The 3D structure of the nickel foam facilitated electron conduction and gas diffusion, and the introduction of Mo increased the number of active catalytic centers and enhanced the catalytic activities. When used in a water splitting system, the voltage at a current density of 10 mA.cm(-2) was only 1.51 V.
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Tingting Yu et al.
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Jinzhou Li et al.
Summary: A collaborative interface optimization strategy was used to prepare a metal-organic framework (MOF) derived heterostructure electrocatalyst (MXene@RuCo NPs), which showed excellent performance in electrocatalytic hydrogen/oxygen evolution reactions. The electrocatalyst exhibited low overpotentials and high current densities, thanks to the introduction of second active sites and the enhancement of the number of active sites by doped Ru. The heterogeneous interfaces of MXene/RuCo NPs in the catalysts also played a significant role in improving the charge transfer rate and reducing the energy barrier of the catalytic reaction.
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Jie Zhu et al.
Summary: In this study, Co5.47N/MoN heterogeneous structure porous nanosheets were successfully designed and synthesized, exhibiting excellent electrocatalytic activity in oxygen evolution reaction (OER) and hydrogen evolution reaction (HER).
APPLIED SURFACE SCIENCE
(2023)
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Kai Chen et al.
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Beibei Sun et al.
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ELECTROCHIMICA ACTA
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Zhixin Dai et al.
Summary: In this paper, the Ni-Co-Fe-Se@NiCo-LDH catalyst was synthesized based on the CoFe-LDH@NiCo-LDH precursor, which exhibited low overpotential and high current density for both OER and HER in alkaline environment. The results showed that increasing the number of metal species only had a slight effect on the electron transfer impedance and did not contribute to the increase in electrochemical surface area. The catalyst showed excellent overall water splitting performance and a low cell voltage.
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Liyan Wang et al.
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JOURNAL OF COLLOID AND INTERFACE SCIENCE
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Borong Lu et al.
Summary: A CoSeP/CoP interface catalyst is synthesized on nickel foam using hydrothermal, solvothermal, and in situ template methods. This catalyst promotes the hydrogen production performance of electrolytic urea and exhibits durable cycle stability. Density functional theory (DFT) confirms that the catalyst can enhance catalytic activity by adsorbing and stabilizing reaction intermediates on its surface.
Article
Engineering, Multidisciplinary
Jibo Jiang et al.
Summary: This study ingeniously designed Mo-doped Mott-Schottky heterostructure by combining metallic MXene and n-type semiconductor NiCoP, which achieved catalyst electron redistribution and reduced the adsorption energy of reaction intermediates. The synthesized 3D triangle plum flower structure Mo-NiCoP@MXene/NF exhibited outstanding performance in hydrogen evolution reaction and oxygen evolution reaction, as well as superb electrolytic stability, suggesting the possibility of developing highly efficient catalysts based on the same design concept.
COMPOSITES PART B-ENGINEERING
(2023)
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Meiling Zhang et al.
Summary: In this study, nanosized Co9Se8 and TiO2 particles were fabricated using a hydrothermal process, followed by the construction of various Co9Se8/TiO2 heterojunctions using a physical solvent evaporation strategy. The photocatalytic H2 evolution experiment demonstrated that the H2 evolution rate over 15%-Co9Se8/TiO2 reached 8282.7 μmol∙g-1∙h-1 under 300 W Xe lamp irradiation, using 20% triethanolamine (TEOA) as the sacrifice agent. This rate was 29.9-fold and 95.8-fold higher than that of pristine TiO2 and Co9Se8, respectively. The enhanced photocatalytic performance was attributed to improved light absorption ability and the formation of S-scheme heterojunctions, which promoted the separation and migration of photo-induced charges.
JOURNAL OF ALLOYS AND COMPOUNDS
(2023)
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Xuliang Lin et al.
Summary: In this work, metal sulfides encapsulated with S/N co-doped carbon were synthesized using a one-step pyrolysis strategy. The encapsulated Co9S8-Ni3S2 heterojunction showed a low overpotential of 200 mV and a high current density of 10 mA cm(-2). It also exhibited excellent stability with only a slight increase in overpotential after a 50-hour chronoamperometric stability test. Density functional theory calculations confirmed the optimized electronic structure and improved OER reaction activity of the Co9S8-Ni3S2 heterojunctions encapsulated with S/N co-doped carbon. This study provides a novel strategy for the construction of highly efficient and sustainable metal sulfide heterojunction catalysts using lignosulfonate biomass as an assistance.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2023)
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Xuedong He et al.
Summary: Achieving high current density is essential for large-scale hydrogen production by water splitting. However, the development of efficient and stable catalysts has been a challenge. In this study, a Pt-induced NiFe layered double hydroxide (LDH) nanosheet was synthesized and demonstrated excellent catalytic performance for both hydrogen evolution reaction (HER) and oxygen evolution reaction (OER). The introduction of Pt to the NiFe LDH structure modulated the electronic structure and improved the catalytic activity and stability. The findings provide a facile strategy for developing catalysts for large current density water splitting.
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Yaxin Li et al.
Summary: In order to meet practical applications, a high-performance and cost-effective (Fe, Ni)2P@Ni2P electrocatalyst was obtained by precise modulation of morphological and electronic properties. The unique porous structure of (Fe, Ni)2P@Ni2P exposes more active sites, and the transfer of electrons from electron-rich Ni2P to electron-negative (Fe, Ni)2P enhances charge transfer efficiency. With ultralow overpotentials, it exhibits excellent catalytic performance and long-term stability in water splitting, providing a new idea for the design of dual-function electrocatalysts for industrial hydrogen production.
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Guiyuan Ma et al.
Summary: Researchers prepared Mn-doped nickel cobalt phosphide (Mn-NiCoP) with nanopins arrays on nickel foam, which exhibited low overpotentials of 148 mV for HER and 266 mV for OER at a high current density. The water splitting performance of Mn-NiCoP as both anode and cathode was 1.69 V and maintained 94% efficiency after 240 hours. By conducting first-principles calculations, it was determined that the synergistic effect of moderate Mn doping and Co alloying contributed to the improvement of both OER and HER performance on Mn-NiCoP. This study provides inspiration for optimizing the OER performance of traditional HER catalysts, facilitating overall water splitting using a single catalyst in the same solution.
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Ming-Yue Ma et al.
Summary: We developed a sulfide-based MoS2/Co1-xS@C hetero-structure for highly efficient electrochemical hydrogen evolution reaction (HER) and oxygen evolution reaction (OER).
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Yu Qi et al.
Summary: The research has successfully developed a high-efficiency and durable non-noble metal-based oxygen evolution reaction (OER) catalyst by growing a CoTe2-NiTe2 heterojunction on CoNi alloy foam, preparing an optimized electrode through hydrothermal method, achieving high OER activity, and demonstrating excellent stability.
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Haotian Zhang et al.
Summary: Efficient and robust bifunctional catalysts are crucial for overall water electrolysis. In this study, a multidimensional hierarchical architecture catalyst was constructed, showing excellent electrocatalytic performance for the hydrogen evolution reaction and oxygen evolution reaction in a water electrolysis device.
ACS SUSTAINABLE CHEMISTRY & ENGINEERING
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Jing Pan et al.
Summary: Design and synthesis of a novel core-shell structured composite material has been demonstrated, showing excellent electrochemical properties and cycling stability in energy storage.
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Lin Tian et al.
Summary: In this study, a facile H2O2-assisted etching method was proposed to fabricate Mo-doped ultrathin Co9Se8@NiSe/NF-X heterojunctions with rich Se vacancies for enhanced electrocatalytic water oxidation. The step-by-step electronic structure modulation by Mo doping and Se vacancy engineering resulted in self-standing Mo-Co9Se8@NiSe/NF-60 heterojunctions that exhibited a high current density and low overpotential for overall water splitting.
Article
Chemistry, Physical
Dongjoon Kim et al.
Summary: In this study, heterostructures of nickel selenide and cobalt-iron layer double hydroxide were prepared and showed enhanced catalytic activity for oxygen evolution reaction and hydrogen evolution reaction through interfacial coupling. These heterostructures exhibited low overpotentials and Tafel slopes, as well as high catalytic activity at a current density of 10 mA·cm(-2). The enhancement of oxygen evolution reaction performance was confirmed by density functional theory calculations. This study provides a strategy for the development of heteronanostructure electrocatalysts for applications such as metal-air batteries and energy storage, and demonstrates their long-term stability.
APPLIED CATALYSIS B-ENVIRONMENTAL
(2022)
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Engineering, Environmental
Ting-Ting Lv et al.
Summary: In this study, a hollow heterostructure Co3V2O8@MnO2 was successfully synthesized by a simple hydrothermal method and an in-situ growth strategy. This material, as a free-standing aqueous zinc-ion batteries cathode, exhibits high conductivity and a hollow structure that can prevent volume change. It also provides sufficient active sites for the electrolyte, resulting in a high discharge capacity and desirable rate performance.
CHEMICAL ENGINEERING JOURNAL
(2022)
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Kaitian Zheng et al.
Summary: This study develops a non-noble metal catalyst for efficient alkaline electrochemical water splitting. The catalyst, a series of crystalline CoMP-decorated amorphous CoM LDH nanomaterials, shows increased catalytic active sites, optimal intermediate adsorption/dissociation capability, and synergistic effects between transition metals, leading to enhanced catalytic performance. The optimized cell assembled with this catalyst exhibits excellent durability and ultralow cell voltages for driving high current densities.
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Jiajun Wang et al.
Summary: Due to the large Gibbs free energy of metal telluride for hydrogen generation, tellurium (Te) based materials are rarely reported as catalysts for overall water splitting. However, through a facile hydrothermal method, stacked flower-like NiTe-NiSe nanosheets have been engineered, bringing transition metal telluride closer to application in the field of clean and renewable energy. The hollow flower-shaped catalyst assembled with nanosheets significantly increases the active surface area, resulting in low overpotentials for hydrogen and oxygen evolution processes.
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Hebing Pei et al.
Summary: Efficient and stable transition metal based electrocatalysts Ni0.85Se-1, Ni0.85Se-2, and Ni0.85Se-3 materials were synthesized via a one-step hydrothermal route. The introduction of carbon nanomaterials as Ni0.85Se/RGO/CNTs nanocomposite further enhanced the catalytic activity. The resulting nanocomposites demonstrated excellent electrocatalytic performance for OER and HER, and could be used as anodes and cathodes in water electrolysis devices with good stability.
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
(2022)
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Donghong Duan et al.
Summary: To solve the environmental pollution and energy crisis, a low-crystallinity and microspherical CoFe-P/NF catalyst was designed and synthesized, which exhibited excellent performance in water splitting. The catalyst showed high activity for both the hydrogen evolution reaction and oxygen evolution reaction, leading to efficient production of hydrogen and oxygen. This study provides a new method for developing cost-effective catalysts for green hydrogen production via water splitting.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2022)
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Jian Chen et al.
Summary: In this study, a hybrid electrocatalyst MoO2-CeOx/NF was synthesized via interfacial engineering, exhibiting outstanding HER and OER activities. It has the potential to achieve high catalytic alkaline overall water splitting and acidic HER performance.
JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY
(2022)
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Jinli Fan et al.
Summary: The study presents a mild construction method for highly efficient and durable electrodes for overall water splitting. The self-supporting electrode, prepared by growing metal-organic framework on carbon cloth and plating with cobalt-boron, exhibits excellent performance in hydrogen and oxygen evolution reactions. It also shows long-term stability in various electrolytes.
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Daoping Cai et al.
Summary: The study successfully designed and synthesized MoSe2-decorated Ni/Co selenide complex hollow arrayed structures, which exhibited excellent performance in aqueous alkaline Zn batteries, demonstrating potential for practical applications.
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Xiaodong Yang et al.
Summary: In this study, crystalline Ag nanoparticles decorated amorphous QLDHs nanosheet arrays were successfully fabricated on Ni foam using a simple method. The material exhibited excellent electrocatalytic performance and structural robustness. In situ Raman spectroscopy revealed the important role of Ag nanoparticles in enhancing the oxidation state of Ni and Fe.
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Kun-Qi Geng et al.
Summary: In this study, a Mo-doped Li-rich layered oxide (LRMO-Mo2.0%) was successfully synthesized and showed enhanced electrochemical performance compared to the pristine counterpart. The improved performance was attributed to the synergic effect of a robust oxygen framework and layered/spinel heterostructure.
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Jian Zeng et al.
Summary: In this study, a series of two-dimensional (2D)/2D Z-scheme systems with interlayer inequivalent were designed and investigated. It was demonstrated that these systems exhibited excellent catalytic activity, environmental stability, and fulfilled the redox potential requirements for water splitting. Additionally, the systems showed enhanced light absorption performance and sliding ferroelectricity, suggesting their promising applications in future nanogenerators. This work provides new insights into energy conversion devices.
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Bin Chen et al.
Summary: A novel bifunctional electrocatalyst consisting of multiple transition metal phosphide nanoclusters and N-doped carbon nanosheets derived from metal-organic frameworks has been successfully synthesized for overall water splitting, showing high HER and OER activities along with excellent stability.
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Abdelhadi El Jaouhari et al.
Summary: The study investigates and optimizes the behavior of selenium vacancies during the OER process using CoNiSe2 films, and finds that an optimized amount of selenium vacancies can significantly enhance the catalytic performance.
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Cheng-Fei Li et al.
Summary: This study demonstrates the efficient design of bifunctional catalysts using doping and vacancy double control strategy for the significant enhancement of hydrogen and oxygen evolution reactions. The Fe-doped Ni5P4/Fe-doped Ni(OH)2 hybrid nanosheets with rich oxygen vacancies show excellent catalytic performances with low overpotentials and cell voltage for water splitting.
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Baojin Chen et al.
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Jin Hu et al.
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Lei Zhang et al.
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Yidong Hu et al.
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