4.7 Article

Two-dimensional fluorescence excitation spectroscopy: A novel technique for monitoring excited-state photophysics of molecular species with high time and frequency resolution

Related references

Note: Only part of the references are listed.
Article Chemistry, Physical

Isolating Pure Donor and Acceptor Signals by Polarization-Controlled Transient Absorption Spectroscopy

Yi Xu et al.

Summary: In this work, a polarization-based strategy is demonstrated and applied to decompose time-resolved optical spectra, allowing for analysis of the electronic structure and energy transfer in a molecular donor-acceptor dyad. By selecting a dyad with orthogonal transition dipole moments and high fluorescence quantum yield, polarization-controlled ultrafast transient absorption spectra can isolate the pure donor and acceptor components of the total signal. This strategy greatly reduces spectral congestion in complex systems, enabling detailed studies of electronic structure and energy transfer.

JOURNAL OF PHYSICAL CHEMISTRY LETTERS (2023)

Review Chemistry, Multidisciplinary

Coherent Two-Dimensional and Broadband Electronic Spectroscopies

Somnath Biswas et al.

Summary: Coherent broadband spectroscopy and two-dimensional electronic spectroscopy have been widely used to investigate ultrafast processes and have made significant progress. These techniques provide important theoretical frameworks and experimental methods for optimizing the photophysical properties of various artificial systems.

CHEMICAL REVIEWS (2022)

Article Multidisciplinary Sciences

Quantum coherent energy transport in the Fenna–Matthews–Olson complex at low temperature

Hong-Guang Duan et al.

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2022)

Review Chemistry, Multidisciplinary

Equation-of-Motion Methods for the Calculation of Femtosecond Time-Resolved 4-Wave-Mixing and N-Wave-Mixing Signals

Maxim F. Gelin et al.

Summary: Femtosecond nonlinear spectroscopy is a crucial method for studying photophysical and photochemical processes, and theoretical support is necessary for analyzing the spectroscopic responses. This article provides a comprehensive review of the spectroscopic equation-of-motion (EOM) methods and their applications in various material systems and spectroscopic signals.

CHEMICAL REVIEWS (2022)

Review Chemistry, Multidisciplinary

Theoretical study of excitation energy transfer and nonlinear spectroscopy of photosynthetic light-harvesting complexes using the nonperturbative reduced dynamics method

Yaming Yan et al.

Summary: This article reviews theoretical studies of photosynthetic light-harvesting complexes using the nonperturbative hierarchical equations of motion (HEOM) approach to simulate EET dynamics and spectroscopic signals. The results demonstrate the effectiveness of the HEOM method in understanding EET pathways and quantum effects in these complexes through simulations.

WILEY INTERDISCIPLINARY REVIEWS-COMPUTATIONAL MOLECULAR SCIENCE (2021)

Article Chemistry, Physical

Computational spectroscopy of complex systems

Thomas L. C. Jansen

Summary: This paper reviews the computational spectroscopy methods that have been developed and applied for infrared and visible spectroscopies in the condensed phase over the past decade, discussing the questions that these methods have allowed answering and current/future challenges and solutions.

JOURNAL OF CHEMICAL PHYSICS (2021)

Article Chemistry, Multidisciplinary

Fluorescence-Detected Pump-Probe Spectroscopy

Pavel Maly et al.

Summary: Fluorescence-detected pump-probe (F-PP) spectroscopy is a new approach to transient spectroscopy that overcomes limitations of traditional methods, providing background-free detection and unique extraction of excited-state dynamics under certain conditions. Despite incoherent detection, F-PP offers time resolution independent of fluorescence lifetime and is broadly applicable to chemical systems in different environments and spectral regimes.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

Article Chemistry, Physical

Broadband visible two-dimensional spectroscopy of molecular dyes

Lars Mewes et al.

Summary: Two-dimensional Fourier transform spectroscopy is a promising technique for studying ultrafast molecular dynamics, providing a more complete picture of dynamics with broadband laser pulses. This experiment presented visible broadband 2D spectra of dye molecules, revealing vibrational coherences and information about structural motion, and allowing for acquisition of 2D spectra with high bandwidth and temporal resolution.

JOURNAL OF CHEMICAL PHYSICS (2021)

Article Chemistry, Physical

Simulation of Nonlinear Femtosecond Signals at Finite Temperature via a Thermo Field Dynamics-Tensor Train Method: General Theory and Application to Time- and Frequency-Resolved Fluorescence of the Fenna-Matthews-Olson Complex

Maxim F. Gelin et al.

Summary: A fully quantum, numerically accurate wave function-based approach for calculating third-order spectroscopic signals of polyatomic molecules and molecular aggregates at finite temperature has been developed. The approach, based on Thermo Field Dynamics (TFD) representation and tensor-train (TT) machinery, efficiently simulates the quantum evolution of systems with many degrees of freedom. The developed approach has been applied to calculate time- and frequency-resolved fluorescence spectra of the Fenna-Matthews-Olson (FMO) antenna complex at room temperature, considering various factors such as finite resolution, orientational averaging, and static disorder.

JOURNAL OF CHEMICAL THEORY AND COMPUTATION (2021)

Article Chemistry, Physical

2D Electronic Spectroscopic Techniques for Quantum Technology Applications

Elisabetta Collini

Summary: 2D electronic spectroscopy techniques are valuable for studying transport processes in artificial nanomaterials and nanodevices, particularly in assessing coherent mechanisms active in the transport of excitation energy towards possible quantum technology applications. The potential impact of 2DES techniques on the field of nanosystems, quantum technologies, and quantum devices is significant, given the promising new applications and rapidly developing technical capabilities.

JOURNAL OF PHYSICAL CHEMISTRY C (2021)

Review Chemistry, Multidisciplinary

Altered relaxation dynamics of excited state reactions by confinement in reverse micelles probed by ultrafast fluorescence up-conversion

Ismael A. Heisler et al.

Summary: Studying chemical reactions in confined media requires consideration of the confinement effect on reaction rate, as well as the understanding of interactions between reactants and confining medium. Ultrafast spectroscopy can be used to measure reaction dynamics, revealing differences in reaction kinetics within the nanoconfined water phase of reverse micelles.

CHEMICAL SOCIETY REVIEWS (2021)

Article Chemistry, Physical

Generalized Huang-Rhys factors for molecular aggregates

Maxim F. Celin et al.

CHEMICAL PHYSICS (2020)

Editorial Material Chemistry, Physical

Interpreting Fluorescence Detected Two-Dimensional Electronic Spectroscopy

Oliver Kuhn et al.

JOURNAL OF PHYSICAL CHEMISTRY LETTERS (2020)

Review Multidisciplinary Sciences

Quantum biology revisited

Jianshu Cao et al.

SCIENCE ADVANCES (2020)

Review Chemistry, Multidisciplinary

Vibrational Spectroscopic Map, Vibrational Spectroscopy, and Intermolecular Interaction

Carlos R. Baiz et al.

CHEMICAL REVIEWS (2020)

Article Chemistry, Physical

Analysis of transient-absorption pump-probe signals of nonadiabatic dissipative systems: Ideal and real spectra

Elisa Palacino-Gonzalez et al.

JOURNAL OF CHEMICAL PHYSICS (2019)

Article Chemistry, Physical

Origin of Unexpectedly Simple Oscillatory Responses in the Excited-State Dynamics of Disordered Molecular Aggregates

Maxim F. Gelin et al.

JOURNAL OF PHYSICAL CHEMISTRY LETTERS (2019)

Review Biochemistry & Molecular Biology

Two-dimensional spectroscopy for non-specialists

Andrius Gelzinis et al.

BIOCHIMICA ET BIOPHYSICA ACTA-BIOENERGETICS (2019)

Article Chemistry, Multidisciplinary

Efficient calculation of open quantum system dynamics and time-resolved spectroscopy with distributed memory HEOM (DM-HEOM)

Tobias Kramer et al.

JOURNAL OF COMPUTATIONAL CHEMISTRY (2018)

Article Chemistry, Multidisciplinary

Identification and characterization of diverse coherences in the Fenna-Matthews-Olson complex

Erling Thyrhaug et al.

NATURE CHEMISTRY (2018)

Review Multidisciplinary Sciences

Recent advances in multidimensional ultrafast spectroscopy

Thomas A. A. Oliver

ROYAL SOCIETY OPEN SCIENCE (2018)

Article Chemistry, Physical

Pulse-shape effects in fifth-order multidimensional optical spectroscopy

Thanh Nhut Do et al.

CHEMICAL PHYSICS (2018)

Review Chemistry, Multidisciplinary

Ultrafast Elementary Photochemical Processes of Organic Molecules in Liquid Solution

Tatu Kumpulainen et al.

CHEMICAL REVIEWS (2017)

Article Chemistry, Physical

Simplified expressions that incorporate finite pulse effects into coherent two-dimensional optical spectra

Thanh Nhut Do et al.

JOURNAL OF CHEMICAL PHYSICS (2017)

Article Chemistry, Physical

Efficient orientational averaging of nonlinear optical signals in multi-chromophore systems

Maxim F. Gelin et al.

JOURNAL OF CHEMICAL PHYSICS (2017)

Review Multidisciplinary Sciences

Using coherence to enhance function in chemical and biophysical systems

Gregory D. Scholes et al.

NATURE (2017)

Article Chemistry, Physical

Anharmonic vibrational effects in linear and two-dimensional electronic spectra

Arpa Galestian Pour et al.

PHYSICAL CHEMISTRY CHEMICAL PHYSICS (2017)

Article Chemistry, Physical

Two-dimensional electronic spectroscopy can fully characterize the population transfer in molecular systems

Jakub Dostal et al.

JOURNAL OF CHEMICAL PHYSICS (2016)

Article Chemistry, Physical

Exciton Structure and Energy Transfer in the Fenna-Matthews-Olson Complex

Erling Thyrhaug et al.

JOURNAL OF PHYSICAL CHEMISTRY LETTERS (2016)

Article Instruments & Instrumentation

Femtosecond broadband fluorescence upconversion spectroscopy: Spectral coverage versus efficiency

Mario Gerecke et al.

REVIEW OF SCIENTIFIC INSTRUMENTS (2016)

Article Multidisciplinary Sciences

Origin of long-lived quantum coherence and excitation dynamics in pigment-protein complexes

Zhedong Zhang et al.

SCIENTIFIC REPORTS (2016)

Review Chemistry, Physical

Experimental Implementations of Two-Dimensional Fourier Transform Electronic Spectroscopy

Franklin D. Fuller et al.

ANNUAL REVIEW OF PHYSICAL CHEMISTRY, VOL 66 (2015)

Article Multidisciplinary Sciences

Vibronic origin of long-lived coherence in an artificial molecular light harvester

James Lim et al.

NATURE COMMUNICATIONS (2015)

Article Chemistry, Physical

Distinguishing Electronic and Vibronic Coherence in 2D Spectra by Their Temperature Dependence

Vaclav Perlik et al.

JOURNAL OF PHYSICAL CHEMISTRY LETTERS (2014)

Article Chemistry, Physical

Transient Grating Photoluminescence Spectroscopy: An Ultrafast Method of Gating Broadband Spectra

Kai Chen et al.

JOURNAL OF PHYSICAL CHEMISTRY LETTERS (2014)

Article Chemistry, Multidisciplinary

Vibronic coherence in oxygenic photosynthesis

Franklin D. Fuller et al.

NATURE CHEMISTRY (2014)

Article Instruments & Instrumentation

Two-dimensional electronic spectroscopy with birefringent wedges

Julien Rehault et al.

REVIEW OF SCIENTIFIC INSTRUMENTS (2014)

Article Chemistry, Physical

Simple Recipes for Separating Excited-State Absorption and Cascading Signals by Polarization-Sensitive Measurements

Maxim F. Gelin et al.

JOURNAL OF PHYSICAL CHEMISTRY A (2013)

Article Multidisciplinary Sciences

Electronic resonance with anticorrelated pigment vibrations drives photosynthetic energy transfer outside the adiabatic framework

Vivek Tiwari et al.

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2013)

Article Multidisciplinary Sciences

Enhancement of Vibronic and Ground-State Vibrational Coherences in 2D Spectra of Photosynthetic Complexes

Aurelia Chenu et al.

SCIENTIFIC REPORTS (2013)

Article Chemistry, Physical

Origin of Long-Lived Coherences in Light-Harvesting Complexes

Niklas Christensson et al.

JOURNAL OF PHYSICAL CHEMISTRY B (2012)

Article Multidisciplinary Sciences

Conformation of self-assembled porphyrin dimers in liposome vesicles by phase-modulation 2D fluorescence spectroscopy

Geoffrey A. Lott et al.

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2011)

Review Chemistry, Multidisciplinary

Coherent Multidimensional Vibrational Spectroscopy of Biomolecules: Concepts, Simulations, and Challenges

Wei Zhuang et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2009)

Article Chemistry, Physical

Fluorescence-detected two-dimensional electronic coherence spectroscopy by acousto-optic phase modulation

Patrick F. Tekavec et al.

JOURNAL OF CHEMICAL PHYSICS (2007)

Article Multidisciplinary Sciences

Two-dimensional spectroscopy at infrared and optical frequencies

Robin M. Hochstrasser

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2007)

Article Multidisciplinary Sciences

Evidence for wavelike energy transfer through quantum coherence in photosynthetic systems

Gregory S. Engel et al.

NATURE (2007)

Article Chemistry, Physical

Transient phenomena in time- and frequency-gated spontaneous emission

MF Gelin et al.

JOURNAL OF PHYSICAL CHEMISTRY A (2005)

Article Multidisciplinary Sciences

Two-dimensional spectroscopy of electronic couplings in photosynthesis

T Brixner et al.

NATURE (2005)

Article Chemistry, Physical

Femtosecond fluorescence spectroscopy by upconversion with tilted gate pulses

LJ Zhao et al.

PHYSICAL CHEMISTRY CHEMICAL PHYSICS (2005)

Article Optics

Noncollinear phase matching in fluorescence upconversion

H Rhee et al.

OPTICS LETTERS (2005)

Article Multidisciplinary Sciences

Femtosecond phase-coherent two-dimensional spectroscopy

PF Tian et al.

SCIENCE (2003)