Journal
CHEMICAL COMMUNICATIONS
Volume 51, Issue 63, Pages 12563-12566Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c5cc04837k
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Funding
- National Basic Research Program of China [2013CB934102, 2011CB808703]
- National Natural Science Foundation of China [21331004, 21301116]
- Shanghai Eastern Scholar Program
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The Kirkendall effect was utilized to synthesize mesoporous silicalite-1 zeolite nanocrystals without the involvement of additional templates. The mesopore size as well as the particle size can be easily controlled by nanoscale Kirkendall growth via significantly reducing the amount of water or tetrapropylammonium hydroxide, which were used in large quantities in conventional methods. The Kirkendall growth method is thus suitable for large-scale synthesis of mesoporous MFI zeolites with very high yields but low cost for practical applications.
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