Journal
CHEMICAL COMMUNICATIONS
Volume 51, Issue 100, Pages 17647-17657Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c5cc07929b
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Funding
- European Research Council under the European Community's Seventh Framework Program (FP7)/ERC Grant [257891]
- Swiss National Science Foundation [155967]
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Monodentate TADDOL-derived phosphoramidites and phosphonites are versatile chiral ligands for enantio-selective Pd(0)-catalysed C-H functionalisations. They enable highly selective cyclisations to access a wide range of chiral carbo-and heterocycles. The high attractiveness of this ligand class consists in their modular structure, allowing for a quick assembly of a library with variable steric properties. Asymmetric C-H functionalisation methods utilising catalytic systems based on Pd(0) complexes and TADDOL-type ligands are presented and aspects of selectivity are discussed.
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