Journal
CHEMICAL COMMUNICATIONS
Volume 51, Issue 19, Pages 4028-4031Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4cc10394g
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Funding
- National Natural Science Foundation of China [21173234, 21133009, U1232203, 21321063]
- Chinese Academy of Sciences [KJCX2.YW.H30]
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Ionic liquid 1-benzyl-3-methylimidazolium bis(trifluoromethylsulfonyl)-imide ([BnMIm][NTf2]) can promote the generation of the (OOH)-O-center dot free radical and thereby efficiently transformed the beta-O-4 lignin model compound 2-phenoxyacetophenone into benzoic acid and phenol using O-2 as the oxidant. Furthermore, the IL-based metal-free catalytic system can also depolymerize other lignin model compounds and organosolv lignin effectively.
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