Journal
CHEMICAL COMMUNICATIONS
Volume 51, Issue 1, Pages 66-69Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4cc08218d
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Funding
- National Science Foundation
- Division of Materials Research [DMR-1262226]
- Swedish Research Council
- Knut and Alice Wallenberg Foundation
- Swedish Energy Agency
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A facile and efficient fabrication approach for homogeneous, crack-free UiO-66 films with exceptionally high crystallinity and tunable thickness on a transparent and conductive glass substrate is reported. Two functionalized species, a catechol ligand and a Fe-2 complex with structural resemblance to the active site of [FeFe] hydrogenase, were introduced into the MOF films via a postsynthetic exchange. Voltammetric studies show the [FeFe] complex in the thinner UiO-66 films (2-5 mu m) can be reduced electrochemically.
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