Journal
CHEMICAL COMMUNICATIONS
Volume 51, Issue 21, Pages 4481-4484Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4cc10029h
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Funding
- Greek Ministry of Education (GSRT)
- European Union through the Excellence 'ARISTEIA' grant [MIS 2961]
- University of Crete - Special Account for Research [KA 3475]
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Mesoporous framework materials comprising lacunary [SiW11O39](8-) polyoxometalate clusters covalently connected by ethane-bridged silsesquioxane linkers were synthesized through a block copolymer-templated cross-linking polymerization of 1,2-bis(triethoxysilyl)ethane in acid solution. These new hybrid materials, which exhibit a high density of catalytic sites, large pore surface and ordered pore structure, are shown to be highly effective in the photocatalytic oxidation of aryl alcohols with molecular oxygen.
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