Journal
CHEMICAL COMMUNICATIONS
Volume 51, Issue 44, Pages 9227-9230Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c5cc01758k
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Funding
- KIT
- Federal Ministry of Education and Research (BMBF) [05K10VKB, 05K13VK2]
- DBU
- ESRF
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The structure of copper sites in Cu-SSZ-13 during NH3-SCR was unravelled by a combination of novel operando X-ray spectroscopic techniques. Strong adsorption of NH3 on Cu, its reaction with weakly adsorbed NO from the gas phase, and slow re-oxidation of Cu(I) were proven. Thereby the SCR reaction mechanism is significantly different to that observed for Fe-ZSM-5.
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