4.7 Article

Oxidative N-heterocyclic carbene catalyzed stereoselective annulation of simple aldehydes and 5-alkenyl thiazolones

Journal

CHEMICAL COMMUNICATIONS
Volume 51, Issue 38, Pages 8134-8137

Publisher

ROYAL SOC CHEMISTRY
DOI: 10.1039/c5cc01587a

Keywords

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Funding

  1. NSFC [21002043, 21272107]
  2. National S&T Major Project of China [2012ZX09504-001-003]
  3. Fundamental Research Funds for the Central Universities [lzujbky-2013-166]

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A highly diastereoselective annulation of simple aldehydes and 5-alkenyl thiazolones, via oxidative NHC catalysis has been developed. This strategy provides facile access to a diverse library of functionalized chiral thiazolo pyrones. Aerobic oxygen can also be applied as a secondary oxidant to avoid the use of stoichiometric organic or inorganic oxidants.

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