Journal
CHEMICAL COMMUNICATIONS
Volume 51, Issue 99, Pages 17540-17543Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c5cc05129k
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Funding
- Science Foundation Ireland for Investigator Project Award [12/IP/1703]
- National University of Ireland
- Cultural Service of the French Embassy in Ireland
- University College Dublin
- Irish Higher Education Authority
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A symmetry breaking spin transition in a Mn(III) complex is reported with three structural phases, a high symmetry high temperature S = 2 phase, an intermediate S = 1/S = 2 ordered phase and an aperiodic low temperature phase with S = 1 cations. The aperiodicity is interpreted as resulting from long-range ordering of the NTf2- anions.
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