Journal
CHEMICAL COMMUNICATIONS
Volume 51, Issue 95, Pages 16988-16991Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c5cc05881c
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Funding
- EPSRC
- University of Nottingham
- ERC
- EPSRC [EP/K038869/1] Funding Source: UKRI
- Engineering and Physical Sciences Research Council [1225332, EP/K038869/1] Funding Source: researchfish
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[Ni(L-1)Fe((BuNC)-Bu-t)(4)](PF6)(2) is a robust (NiFeII)-Fe-II complex that undergoes a reversible one-electron reduction. Spectroscopic and theoretical studies show that [Ni(L-1)Fe((BuNC)-Bu-t)(4)](+) is an unprecedented (NiFeII)-Fe-I species that reproduces the electronic configuration of the Ni-L state of the [NiFe] hydrogenases.
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