Accelerated Catalytic Ozonation in a Mesoporous Carbon-Supported Atomic Fe-N4 Sites Nanoreactor: Confinement Effect and Resistance to Poisoning

Review Chemistry, Inorganic & Nuclear

Progress in metal-organic-framework-based single-atom catalysts for environmental remediation

Wei Qu et al.

Summary: This review summarizes the synthesis methods and applications of MOF-based single-atom catalysts (SACs) in environmental remediation and proposes future development directions.

COORDINATION CHEMISTRY REVIEWS (2023)

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Article Engineering, Environmental

Layered Double Hydroxide Catalysts for Ozone Decomposition: The Synergic Role of M2+ and M3+

Zhisheng Wang et al.

Summary: The study achieved excellent activity and stability in catalytic ozone decomposition by preparing NiFe-LDH materials, which showed better performance compared to LDH materials containing other metal elements.

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2022)

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Article Engineering, Environmental

Single-Atom Cobalt Incorporated in a 2D Graphene Oxide Membrane for Catalytic Pollutant Degradation

Xuanhao Wu et al.

Summary: A new graphene oxide-based membrane architecture was developed to efficiently degrade a specific pollutant using cobalt catalysts loaded in nanoscale pore walls. The use of a unique synthesis procedure enabled the dispersion of cobalt atoms uniformly, maintaining the membrane's structure and functionality. This study presents a critical advancement in developing catalytic membranes that combine membrane filtration and advanced oxidation processes in a more efficient single-step treatment.

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2022)

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Article Engineering, Environmental

Enhanced Catalytic Ozonation for Eliminating CH3SH via Stable and Circular Electronic Metal-Support Interactions of Si-O-Mn Bonds with Low Mn Loading

Dingren Ma et al.

Summary: This study demonstrates the catalytic ozonation of methyl mercaptan using an Si-O-Mn-based electronic metal-support interaction (EMSI) coordination structure. The results show that this catalyst effectively degrades methyl mercaptan and generates CO2/SO42- as products. Furthermore, the study highlights the importance of the EMSI coordination structure in improving catalytic performance.

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2022)

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Article Chemistry, Physical

Realizing a redox-robust Ag/MnO2 catalyst for efficient wet catalytic ozonation of S-VOCs: Promotional role of Ag(0)/Ag(I)-Mn based redox shuttle

Chun He et al.

Summary: A novel process for S-VOCs degradation using wet scrubbing coupled with catalytic ozonation was developed, and Ag/R-MnO2 catalyst exhibited superior performance in wet catalytic ozonation process. The efficient electron replenishing interaction between Ag(0)/Ag(I) and multivalent R-MnO2, efficient O3 activation through oxygen vacancies-rich R-MnO2, and enhanced mass diffusion in wet scrubbing process contribute to the excellent performance.

APPLIED CATALYSIS B-ENVIRONMENTAL (2022)

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Article Engineering, Environmental

Insights into the Mechanism of Ozone Activation and Singlet Oxygen Generation on N-Doped Defective Nanocarbons: A DFT and Machine Learning Study

Guangfei Yu et al.

Summary: In this study, the O-3 activation mechanism and active sites of N-doped defective nanocarbon catalysts in catalytic ozonation were systematically investigated using density functional theory calculations. The results revealed the decomposition mechanism of O-3 and identified the N4V2 system as the most active catalyst. Furthermore, machine learning models were applied to correlate the O-3 activation activity with catalyst surface properties, with XGBoost performing the best and the condensed dual descriptor being the most important feature.

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2022)

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Article Engineering, Environmental

Biotemplate Fabrication of Hollow Tubular CexSr1-xTiO3 with Regulable Surface Acidity and Oxygen Mobility for Efficient Destruction of Chlorobenzene: Intrinsic Synergy Effect and Reaction Mechanism

Yukun Sun et al.

Summary: This study demonstrates the synthesis of ternary CexSr1-xTiO3 catalysts with elegant chlorine resistance and organic byproduct inhibition capability using the hollow tubular-structured fruit hair of Platanus as the biotemplate. The catalysts exhibit high concentration of oxygen vacancy and acid sites, promoting C-Cl cleavage and desorption of inorganic chlorine. Additionally, the tubular structure accelerates the flow rate of chlorobenzene and reduces the residence time of byproducts.

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2022)

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Article Chemistry, Physical

Magnetic double-core@shell MnO2@NiFe@DE as a multifunctional scavenger for efficient removal of tetracycline, anionic and cationic dyes

Xingjian Dai et al.

Summary: In this study, magnetic MnO2@NiFe@DE nanocomposites with double-core@shell structures were successfully synthesized via a two-step hydrothermal method. The nanocomposite exhibited excellent performance in removing pollutants from wastewater, especially in low pH solutions. The effects of solution pH, adsorption time, and contaminant concentration on the performance of the nanocomposite were investigated, and physical adsorption and oxidation were identified as the main mechanisms for contaminant removal. The use of permanent magnets enabled sustainable recovery of the adsorbent and the adsorbed substances. Overall, the synthesized nanocomposite is a multifunctional material with high removal efficiency, low cost, and easy separation, making it a promising solution for organic wastewater treatment, particularly in low pH conditions.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2022)

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Article Chemistry, Multidisciplinary

Interstitial Atomic Bi Charge-Alternating Processor Boosts Twofold Molecular Oxygen Activation Enabling Rapid Catalytic Oxidation Reactions at Room Temperature

Qiyu Lian et al.

Summary: This study demonstrates that interstitial atomic Bi anchored in the lattice interstice of MnO2 can boost the catalytic oxidation reactions by triggering an alternative twofold O-2 activation, weakening the O-2 dissociation energy barrier by reconstructing the local charge landscape and elongating the O-O bond length.

ADVANCED FUNCTIONAL MATERIALS (2022)

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Article Engineering, Environmental

Engineering Platinum Catalysts via a Site-Isolation Strategy with Enhanced Chlorine Resistance for the Elimination of Multicomponent VOCs

Ruyi Gao et al.

Summary: This study demonstrates the catalytic roles of a bifunctional catalyst with an atomic-scale metal/oxide interface. The catalyst exhibits strong resistance to chlorine at low temperatures and excellent catalytic stability in the oxidation of multicomponent volatile organic compounds (VOCs).

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2022)

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Article Chemistry, Multidisciplinary

Ultrafine Ruthenium Clusters Shell-Embedded Hollow Carbon Spheres as Nanoreactors for Channel Microenvironment-Modulated Furfural Tandem Hydrogenation

Zhihao Yu et al.

Summary: This study presents a metal pre-chelating assisted assembly strategy to synthesize Ru@Shell-HCSs nanoreactors with preferred catalytic microenvironments for efficient hydrogenation of biomass-derived furfural. The channel-embedding structure enhances the electron-deficient property of ultrafine ruthenium clusters, leading to an accelerated tandem hydrogenation progression for enhanced 2-methylfuran generation.

SMALL (2022)

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Article Multidisciplinary Sciences

Angstrom-confined catalytic water purification within Co-TiOx laminar membrane nanochannels

Chenchen Meng et al.

Summary: The global shortage of freshwater and inadequate access to clean water have led to the development of efficient technologies for water purification. Heterogeneous catalysis is a highly promising solution and sub-nanometer-confined reactions have been found to achieve unprecedented reaction rates. This study successfully demonstrates the degradation of water contaminants at an incredibly fast rate using a two-dimensional laminate membrane assembled from cobalt-doped titanium oxide nanosheets.

NATURE COMMUNICATIONS (2022)

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Article Chemistry, Physical

Confining intermediates within a catalytic nanoreactor facilitates nitrate-to-ammonia electrosynthesis

Wenxi Qiu et al.

Summary: This work demonstrates the incorporation of CuOx active species into a TiO2 nanotube reactor for selective electrocatalytic nitrate reduction reactions. The diffusion of the intermediate NO2- is hindered due to the nanoconfined space, leading to a high faradaic efficiency and conversion rate of nitrate to ammonia. Theoretical insights further support the understanding of the surface and interface interactions.

APPLIED CATALYSIS B-ENVIRONMENTAL (2022)

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Article Chemistry, Physical

2D-3D magnetic NiFe layered double hydroxide decorated diatomite as multi-function material for anionic, cationic dyes, arsenate, and arsenite adsorption

Xingjian Dai et al.

Summary: A novel magnetic nano adsorbent was synthesized by decorating a magnetic two-dimensional layered double hydroxides nanosheet onto three-dimensional diatomite. This adsorbent exhibited excellent adsorption performance for anionic and cationic dyes, As(V), and As(III) due to the synergistic effect of diatomite and NiFe LDH. The study also investigated the influence of pH, concentrations, contact time, and temperature on the adsorption properties, providing insights into the adsorption mechanism. This research provides a direction for the development of low-cost, magnetic multifunctional nano adsorbents for practical wastewater purification.

APPLIED CLAY SCIENCE (2022)

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Article Engineering, Environmental

Evaluation of the Flexibility for Catalytic Ozonation of Dichloromethane over Urchin-Like CuMnOX in Flue Gas with Complicated Components

Li Xiang et al.

Summary: The study evaluated the poisoning effect of complex components in practical gas on DCM catalytic ozonation and found that Ca/Pb loading weakens catalytic performance, while the presence of As leads to excessive acidity and the formation of byproducts. The catalytic ozonation of DCM displays a distinctive advantage in metal antipoisoning.

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2022)

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Article Engineering, Environmental

Tuning the Micro-coordination Environment of Al in Dealumination Y Zeolite to Enhance Electron Transfer at the Cu-Mn Oxides Interface for Highly Efficient Catalytic Ozonation of Toluene at Low Temperatures

Qi Shao et al.

Summary: In this study, the micro-coordination environment of Al in commercial Y zeolite was regulated by a specific dealumination method to prepare the optimized Cu-Mn/DY catalyst, which exhibited excellent performance at low temperature with around 95% removal of Toluene. The catalyst also showed stability in high-humidity conditions and long-term reactions due to the more active oxygen vacancies and acidic sites.

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2022)

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Article Engineering, Environmental

Unraveling the Synergistic Reaction and the Deactivation Mechanism for the Catalytic Degradation of Double Components of Sulfur-Containing VOCs over ZSM-5-Based Materials

Rui Tian et al.

Summary: This study provides insights into the competitive adsorption, catalysis, reaction, and deactivation mechanisms for decomposing double components of sulfur-containing VOCs, with lanthanum-modified ZSM-5 showing potential environmental application due to its excellent stability and water resistance.

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2022)

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Article Chemistry, Multidisciplinary

Facile synthesis of a 2D multilayer core-shell MnO2@LDH@MMT composite with a nanoflower shape for electromagnetic wave absorption

Quan Zhou et al.

Summary: Manganese dioxide@NiFe layered double hydroxide@montmorillonite (MNFM) with a nanoflower-like two-dimensional layered core-shell construction has been successfully synthesized using a two-step hydrothermal method. The influences of structure and composition on its electromagnetic wave (EW) absorption characteristics were discussed. MNFM with different thicknesses exhibited excellent performance, showing promising potential as a material for electromagnetic wave absorption.

CRYSTENGCOMM (2022)

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Article Engineering, Environmental

Engineered Nanoconfinement Accelerating Spontaneous Manganese-Catalyzed Degradation of Organic Contaminants

Shuo Zhang et al.

Summary: Manganese(III/IV) oxide minerals have been found to degrade organic pollutants in nature, but the kinetics are too slow for practical water treatment processes. By confining nanoscale Mn3O4 particles to 3-5 nm, the degradation kinetics of pollutants can be significantly accelerated, nearly 3 orders of magnitude faster than in the unconfined bulk phase. The acceleration is attributed to the increased surface area of catalysts exposed to the reaction and the local proton concentration at the Mn3O4 surface.

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2021)

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Article Engineering, Environmental

Enhanced Catalytic Ozonation for Eliminating CH3SH via Graphene-Supported Positively Charged Atomic Pt Undergoing Pt2+/Pt4+ Redox Cycle

Yajing Huang et al.

Summary: The study successfully constructed atomically dispersed Pt catalysts with electronic metal-support interaction (EMSI), achieving efficient catalytic ozonation for CH3SH degradation by supporting positively charged Pt atoms on graphene. The circulation between Pt2+ and Pt4+ is essential for maintaining stable catalytic activity over 12 hours.

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2021)

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Article Chemistry, Multidisciplinary

Nanocapillarity and Nanoconfinement Effects of Pipet-like Bismuth@Carbon Nanotubes for Highly Efficient Electrocatalytic CO2 Reduction

Wenjun Zhang et al.

Summary: By semi-filling bismuth nanorods into nitrogen-doped carbon nanotubes, a highly selective electrocatalytic CO2 reduction reaction was achieved with improved activity and stability of the catalyst.

NANO LETTERS (2021)

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Enhanced Organic Photocatalysis in Confined Flow through a Carbon Nitride Nanotube Membrane with Conversions in the Millisecond Regime

Yajun Zou et al.

Summary: The use of a free-standing and flow-through carbon nitride nanotube (CNN) membrane with a pore diameter of 40 nm for confined photocatalytic reactions has shown improved performance compared to bulk reactions, achieving a higher catalytic turnover frequency. This nanoconfined catalysis strategy allows for quantitatively assessing the photocatalytic performance in spatially isolated nanoreactors, providing crucial insights on catalysis in such environments and potentially gaining a fundamental understanding of complex chemical processes.

ACS NANO (2021)

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Article Engineering, Environmental

3D graphene-like zeolite-templated carbon with hierarchical structures as a high-performance adsorbent for volatile organic compounds

Nam Sun Kim et al.

Summary: The study compared the dynamic adsorption of benzene on different carbon materials and found that hierarchical mesoporous/microporous beta zeolite-templated carbon (HBTC) had higher adsorption capacity and breakthrough time for benzene compared to commercial activated carbon (AC) and solely microporous beta zeolite-templated carbon (BTC). Introducing mesoporosity into microporous BTC to form a hierarchically mesoporous/microporous structure solved the diffusion problem and improved benzene adsorption performance. The HBTC showed promising potential for volatile organic compound (VOC) adsorption with higher adsorption capacity and better performance at 10% breakthrough compared to other tested carbons.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Chemistry, Multidisciplinary

Ozone Decomposition by a Manganese-Organic Framework over the Entire Humidity Range

Zhi-Bing Sun et al.

Summary: Ground-level ozone is a major airborne pollutant harmful to human health and ecosystems. The design of high-performance ozone elimination catalysts suitable for varying air compositions, especially water vapor content, remains challenging. ZZU-281, a new manganese-based metal organic framework, shows efficient ozone decomposition over a wide humidity range and possesses unique open channels and water stability.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2021)

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Article Multidisciplinary Sciences

Thermal resistance effect on anomalous diffusion of molecules under confinement

Jiamin Yuan et al.

Summary: Contrary to the general trend, the movement of long-chain molecules slows at higher temperatures under confinement due to the thermal resistance effect. This phenomenon limits molecular transportation in nanoscale channels, as confirmed by zero length column experiments. This study contributes to our understanding of anomalous diffusion and its mechanisms in confined systems.

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2021)

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Article Chemistry, Multidisciplinary

On-Surface Polymerization of In-Plane Highly Ordered Carbon Nitride Nanosheets toward Photocatalytic Mineralization of Mercaptan Gas

Fangsong Guo et al.

Summary: 2D carbon nitride nanosheets with in-plane highly ordered structure (PCNNs-IHO) are successfully prepared by on-surface polymerization of melamine on NaCl crystal surface at elevated temperatures. The NaCl crystals with relative high surface energy facilitate the adsorption and activation of melamine to undergo condensation reaction, and also function as unique substrates to orientate the assembly of 2D nanosheet structure. NaCl acts as a reactant to provide Na+ doping into carbon nitride matrix, affording PCNNs-IHO with robust structural base sites. PCNNs-IHO exhibits superior photocatalytic performance toward CH3SH mineralization under visible light irradiation.

ADVANCED MATERIALS (2021)

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Article Engineering, Environmental

Self-supported bifunctional electrocatalysts with Ni nanoparticles encapsulated in vertical N-doped carbon nanotube for efficient overall water splitting

Yu Cheng et al.

Summary: The study developed a Ni nanoparticle array bifunctional electrocatalyst NCNT-NP@NF through solid-state diffusion method, demonstrating outstanding performance and long-term stability in water splitting process, with enhanced electrocatalytic kinetics.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Engineering, Environmental

Membrane-Confined Iron Oxychloride Nanocatalysts for Highly Efficient Heterogeneous Fenton Water Treatment

Shuo Zhang et al.

Summary: The study achieved the degradation of organic pollutants in complex water matrices by loading iron oxychloride catalysts into the pores of a ceramic ultrafiltration membrane. The membrane, with a pore size that excludes natural organic matter, selectively exposed smaller organics to hydroxyl radicals, effectively inhibiting the degradation of organic pollutants.

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2021)

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Bifunctional Fe for Induced Graphitization and Catalytic Ozonation Based on a Fe/N-Doped Carbon-Al2O3 Framework: Theoretical Calculations Guided Catalyst Design and Optimization

Changpei Ouyang et al.

Summary: Heterogeneous catalytic ozonation is considered a viable technology for advanced wastewater treatment, and Fe/N-doped CAF showed promising results in treating secondary effluent. Theoretical calculations guided catalyst optimization and provided a new direction for designing ozonation catalysts. Fe/N-doped CAF demonstrated great potential for practical applications.

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Environmental Applications of Engineered Materials with Nanoconfinement

Shuo Zhang et al.

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Facet Engineered α-MnO2 for Efficient Catalytic Ozonation of Odor CH3SH: Oxygen Vacancy-Induced Active Centers and Catalytic Mechanism

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Cage-confinement of gas-phase ferrocene in zeolitic imidazolate frameworks to synthesize high-loading and atomically dispersed Fe-N codoped carbon for efficient oxygen reduction reaction

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Self-Accelerating Interfacial Catalytic Elimination of Gaseous Sulfur- Containing Volatile Organic Compounds as Microbubbles in a Facet- Engineered Three-Dimensional BiOCl Sponge Fenton-Like Process

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Accelerated Catalytic Ozonation in a Mesoporous Carbon-Supported Atomic Fe-N4 Sites Nanoreactor: Confinement Effect and Resistance to Poisoning

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