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JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
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Summary: In this study, we developed an in situ assembly growth method to control the growth of NiTCNQ on the surface of graphdiyne (GDY). We achieved a catalytic system with multiple charge transfer by controlling the growth of NiTCNQ on GDY. The resulting catalyst showed high conductivity and typical semiconductor characteristics, which contributed to its high catalytic activity.
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Jiahao Ma et al.
Summary: By engineering the surface of the bimetallic Ni/Co-MOFs with hydrogen-substituted graphdiyne, a hybrid nanoarray with a multifunctional interface has been achieved for the synthesis of ammonia. The NiCoBDC@HsGDY nanoarray promotes both the deoxygenation and hydrogenation reactions, resulting in high NH3 yield rates. When applied in a galvanic Zn-NO3- battery, it exhibits a high power density, indicating its potential in aqueous Zn-based batteries.
Review
Chemistry, Multidisciplinary
Jian Li et al.
Summary: This article first summarizes the prospect of graphdiyne (GDY) as a promising photocatalytic material for solar energy conversion, with direct band gap, excellent carrier mobility, and uniform pores. Then, it elaborates on the construction and progress of GDY-based photocatalysts for solar energy conversion, including H2 evolution reaction, CO2 reduction reaction, and N2 reduction reaction. Finally, the challenges and perspectives in developing GDY-based photocatalysts for solar fuel production are discussed.
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Xuchen Zheng et al.
Summary: Efficient production of ammonia by reducing nitrates at room temperature and ambient pressure is a promising alternative to the Haber-Bosch process that can effectively overcome water pollution issues. The construction of a sp-carbon-metal-carbon interface greatly enhances charge transfer ability and electrical conductivity, leading to high selectivity, activity, and stability in the catalytic system.
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Xuechao Li et al.
Summary: In this study, the acetylenic homocoupling reaction of polarized terminal alkynes on Au(111) was examined using bond-resolved scanning probe microscopy. The replacement of benzene with pyridine moieties effectively inhibited the cyclotrimerization pathway and promoted linear coupling to produce well-aligned N-doped graphdiyne nanowires. Density functional theory calculations revealed that the pyridinic nitrogen modification significantly influenced the coupling motifs at the initial C-C coupling stage (head-to-head vs head-to-tail), which determined the preference of linear coupling over cyclotrimerization.
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
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Summary: Realizing efficient hydrogenation of N2 molecules in the electrocatalytic nitrogen reduction reaction is crucial but rarely reported. A new study presents a highly efficient electrocatalyst with a hydrogen radical-transferring mechanism, which can greatly reduce the potential and maintain high activity and selectivity in NRR.
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
(2023)
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Chao Zhang et al.
Summary: We report a bimetal atomic catalyst of CuEr-GDY featuring atomically dispersed Cu and Er atoms on crystalline graphdiyne for converting CO2 into sustainable fuel. The CuEr-GDY can efficiently separate electron-hole pairs for water oxidation and CO2 activation/reduction, as well as promote CO2/H2O adsorption and CO desorption. This heteroatomic catalyst exhibits high catalytic activity with a reaction selectivity of 97.6% and suppressed competitive hydrogen evolution reaction, achieving a CO yield of 181.04 lmol g-1 h-1 under ambient conditions.
Article
Multidisciplinary Sciences
Shuanglei Xie et al.
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PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA
(2023)
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Danyan Zhang et al.
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NATIONAL SCIENCE REVIEW
(2023)
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Zhiqiang Zheng et al.
Summary: A new type of zerovalent atom catalysts comprised of zerovalent Ir atoms highly dispersed and anchored on graphdiyne (Ir-0/GDY) is developed. The catalyst can selectively and efficiently produce styrene oxides (SO) by electro-oxidizing styrene (ST) in aqueous solutions at ambient conditions. The incomplete charge transfer between Ir-0 and GDY plays a crucial role in enhancing the electron exchange and achieving the selective epoxidation of ST to SO.
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(2023)
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Xuchen Zheng et al.
Summary: Graphdiyne (GDY), a two-dimensional all-carbon network with sp/sp(2)-hybridized structure, has shown great potential for innovation and development in various fields. GDY has attracted extensive attention from scientists due to its controlled growth, chemical and physical properties, and mechanisms that differ from traditional carbon materials. It has become one of the frontiers of chemistry and materials science and has generated numerous research achievements in the fundamental and applied study of carbon materials. The applications of GDY in catalysis, energy storage, photoelectronic, biomedicine, environmental science, life science, detectors, and material separation are comprehensively introduced in this review.
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Jiahao Ma et al.
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Yan Fang et al.
Summary: An iron vacancy-rich ferroferric oxide/graphdiyne heterostructure was designed and fabricated for high-efficiency electrocatalytic nitrogen fixation to ammonia. Experimental and theoretical results show promising electrocatalytic performances with high ammonia yield and Faradaic efficiency, as well as long-term stability in neutral electrolytes. The proposed cationic vacancy activation strategy has strong general guiding significance for the design of new efficient electrocatalysts.
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Haiyuan Zou et al.
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ADVANCED FUNCTIONAL MATERIALS
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Xiaoyu Luan et al.
Summary: Directly extracting hydrogen energy from water to achieve sustainable hydrogen energy generation is a major step towards a zero-pollution hydrogen-fueled economy. The new concept of hydrogen energy conversion allows for the efficient generation of electric energy by reducing nitrate to ammonia. The hydrogen conversion device demonstrates high capacity and efficiency, surpassing lithium and battery solutions.
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(2022)
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Guodong Shi et al.
Summary: By anchoring Cu single atoms on graphdiyne, we successfully constructed a Cu-C bond, which promotes the formation of CH4 during CO2 reduction and enhances catalytic performance.
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(2022)
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Zhiqiang Zheng et al.
Summary: This study focuses on the electrochemical synthesis of ammonia under environmental conditions. By synthesizing independent dispersed zero-valent copper atomic catalysts, the researchers achieved high ammonia yield and efficiency. The catalyst showed excellent performance in ammonia production and maintained its catalytic activity over multiple cycles.
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Fei Zheng et al.
Summary: The novel CRISPR-empowered SPR sensing platform developed in this study combines CRISPR technology with SPR sensor technology to enable rapid, precise, sensitive, and specific detection of target gene sequences.
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Lan Hui et al.
Summary: The Pt/NGDY catalyst prepared using N-doped graphdiyne (NGDY) shows excellent activity, high pH adaptability, and high CO tolerance for methanol oxidation reaction (MOR), making it a promising alternative to noble metal catalysts.
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Ya Kong et al.
Summary: In this study, GDY thin films were successfully synthesized using a Cu(II)-TMEDA catalyst at a liquid/liquid interface, achieving rapid and controllable synthesis. The prepared GDY films exhibited controllable thickness and large-scale uniform morphology. Moreover, the as-grown GDY films showed excellent photothermal conversion efficiency and synergistic antibacterial effect.
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Summary: The proposed physical clipping strategy of targeting chemical bonds in graphdiyne (GDY) enhances the delocalization degree of π electrons, leading to top-ranking electrocatalytic performance without intentionally introducing external decoration. This approach provides a universal prescription for pushing the limits of delocalization degree in metal-free catalysts, offering insights for the rational design of efficient catalytic materials.
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Yang Gao et al.
Summary: Seawater electrolysis is an important direction for the development of hydrogen energy conversion, and achieving high selectivity, activity, and stability in seawater electrolysis reactions is the key challenge. In this report, the construction of heterostructures GDY/RhOx/GDY demonstrated high-performance overall seawater electrolysis.
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA
(2022)
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Yang Gao et al.
Summary: This study reports the facile synthesis of well-defined Rhodium nanocrystals with high-density atomic steps in aqueous solution. The experimental results demonstrate the excellent electrocatalytic performance and high stability of the synthesized catalyst.
NATURE COMMUNICATIONS
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Feng He et al.
Summary: Graphdiyne (GDY) has shown transformative characteristics in various fields, promoting significant progress in fundamental and applied research. Its unique electronic and chemical structure has rapidly advanced GDY science and produced exciting results in energy-related areas such as membrane sciences, catalysis, energy storage, and conversion.
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Zhiqiang Zheng et al.
Summary: This review systematically summarizes the new progress in Graphdiyne (GDY), highlighting its applications in energy, catalysis, and photoelectric devices, and discussing the potential advantages and challenges in this field.
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Yan Fang et al.
Summary: Graphdiyne (GDY), as a new member of carbon allotropes, possesses unique chemical and electronic structures and has found applications in energy, catalysis, environmental science, and electronic devices. It has been recognized for its scientific value and development potential.
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Huidi Yu et al.
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