Journal
CHEMICAL COMMUNICATIONS
Volume 51, Issue 100, Pages 17772-17774Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c5cc06487b
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Funding
- Ministry of Education of China [IRT1225]
- National Natural Science Foundation of China [21362002, 41465009, 81260472]
- State Key Laboratory Cultivation Base for the Chemistry and Molecular Engineering of Medicinal Resources
- Ministry of Science and Technology of China [CMEMR2014-A02, CMEMR2012-A20]
- Bagui Scholar Program of Guangxi
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A novel and efficient approach to the synthesis of 2,5-disubstituted oxazoles is developed via a 1,3-dipolar cycloaddition/ring cleavage/1,2-H migration/denitrogenation/copper-catalyzed aerobic oxidative dehydrogenative cyclization cascade. The desired products can be obtained from readily available aromatic terminal alkenes and azides employing air as the oxidant under mild conditions, and it offers an attractive alternative method for the synthesis of oxazole derivatives.
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