4.7 Article

Synergistic effects of silica aerogels and SDS nanofluids on CO2 sequestration and enhanced oil recovery

Journal

CHEMICAL ENGINEERING JOURNAL
Volume 476, Issue -, Pages -

Publisher

ELSEVIER SCIENCE SA
DOI: 10.1016/j.cej.2023.146589

Keywords

Silica aerogel; CCUS; Enhanced oil recovery; CO2 storage

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This study explores the combined application of hydrophobic silica aerogels and SDS to enhance CO2 storage capacity and oil recovery. Experimental data and molecular dynamics simulations demonstrate the increased solubility and adsorption of CO2 in silica aerogel-SDS nanofluids. Core flooding experiments and two-dimensional tests show improved CO2 trapping efficiency and oil recovery using the nanofluids compared to SDS solutions. The combined agents present an effective approach for geological CO2 storage and EOR optimization.
This study explores the combined application of hydrophobic silica aerogels and SDS to enhance CO2 storage capacity and oil recovery. Experimental data highlighted a marked increase in CO2 solubility within silica aerogel-SDS nanofluids compared to brine and SDS solutions. Molecular dynamics simulations revealed CO2 adsorption into nanopores. Silica aerogel nanoparticles extended CO2 foam half-life by 6 % versus 62 % decline for sole SDS foam from 30 to 140 degrees C. Adjusting the SDS to nanoparticle ratio affects foam properties, with a ratio of 1.5 yielding optimal results. Core flooding experiments demonstrated a 75 % rise in CO2 trapping efficiency using the nanofluids over SDS solutions. Two-dimensional tests showed aerogel-SDS foam surpassed SDS foam flooding by 12 % incremental oil recovery in upper layers, attributed to enhanced profile control. The combined agents present an effective approach for geological CO2 storage and EOR optimization.

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