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Summary: This article provides a comprehensive review on the development of cost-effective and environmentally friendly energy storage devices, focusing on the application of environmentally viable water-in-salt electrolytes in high-performance energy storage devices. The water-in-salt electrolyte exhibits a wide electrochemical stability window, high safety, non-flammability, and superior electrochemical performance compared to conventional salt-in-water electrolytes. The article systematically reviews the strategic application of water-in-salt electrolytes in rechargeable metal-ion batteries and supercapacitors with potentially improved electrochemical performance, and discusses the unique advantages, future prospects, and challenges of water-in-salt electrolytes.
JOURNAL OF ENERGY CHEMISTRY
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Yu Zhang et al.
Summary: Environmental pollution is a global issue that has attracted widespread attention. Metal-organic frameworks (MOFs) have shown promise in the removal of environmental contaminants, but their efficiency needs improvement. Researchers have been modifying MOFs to introduce new functionalities for better pollutant removal. This review highlights the progress in functional modification of MOFs for air and water pollutant treatment, discussing their classification, modification approaches, applications, stability, and future trends.
CHEMICAL ENGINEERING JOURNAL
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Anna A. Lysova et al.
Summary: This study thoroughly investigated the adsorption and separation of light saturated hydrocarbons (methane, ethane, and propane) on a series of metal-organic frameworks. The impact of the size and nature of the glycol moiety on the adsorption parameters was revealed. The studied metal-organic frameworks showed exceptional performance in the practical separation of natural gas or other relevant mixtures of light alkanes.
CHEMICAL ENGINEERING JOURNAL
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Mohan Gopalakrishnan et al.
Summary: Rechargeable aqueous zinc-ion batteries (AZIBs) have gained much interest due to their high energy density, safety, and low cost. However, issues such as anode side reactions, passivation, corrosion, hydrogen evolution, and Zn dendrite growth continue to hinder their widespread application. This review presents metal-organic frameworks (MOFs) as potential solutions to these problems by enhancing the performance of Zn anode materials, electrolytes, and electrolyte additives through their porous structure and active sites. The review also proposes directions for the rational design of MOF-based Zn anodes and understanding the mechanisms affecting Zn2+ solvation in high-performance AZIBs, aiming to extend the cycling lifetime and promote the commercialization of AZIBs.
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Ha Huu Do et al.
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INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
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Li Yan et al.
Summary: The problem of bacterial resistance to antibiotics is becoming increasingly serious, and the development of new antibiotics is much slower than the development of antibiotic resistance in pathogenic bacteria. To overcome antibiotic resistance, new therapeutic strategies need to be sought, and new materials such as metal organic frameworks may be potential candidates.
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NATIONAL SCIENCE REVIEW
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COMPOSITES PART B-ENGINEERING
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Rupam Sahoo et al.
Summary: This article introduces the research progress of metal-organic frameworks and coordination polymers as solid-state proton conductors, and discusses key examples of proton conduction driven by coordinated water molecules. These materials have promising applications due to their structural superiority and wide range of proton conductivity.
ACS ENERGY LETTERS
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George Shimizu et al.
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ACS ENERGY LETTERS
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Prakas Samanta et al.
Summary: In this study, an asymmetric-bipolar Zn-ion battery (ZiB) was proposed, in which the cathode and anode work at different pHs to improve energy density. Efficiency of Zn2+ accepting the host was enhanced through modification of the MoS2 layer. Investigation on charge storage mechanisms was conducted.
ACS APPLIED ENERGY MATERIALS
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Rupam Sahoo et al.
Summary: Efforts have been made to separate CO2 from flue gas and biogas using nonthermal-based separations, such as adsorption-based or membrane-separation technology employing metal-organic frameworks (MOFs). This review summarizes the strategies, performance parameters, and molecular-level mechanisms of such separations, and offers critical insights and future recommendations for further development of MOF materials as flue and biogas separators.
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Summary: Due to the excessive consumption of nonrenewable resources, the exploration of effective and durable materials for sustainable energy conversion and storage is highly sought after. Metal-organic frameworks (MOFs) are a new class of hybrid materials that have gained traction in energy-related fields. Vanadium-MOFs (V-MOFs) possess unique structural characteristics and satisfactory electrochemical properties. Furthermore, V-MOFs-derived materials also exhibit superior electrical conductivity and stability when used as electrocatalysts and electrode materials. This review summarizes the research progress and potential applications of V-MOFs and their derivatives in electrochemical energy conversion and storage. Future possibilities and challenges in terms of design and synthesis are also discussed.
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Anh N. Hong et al.
Summary: Pore space partition (PSP) concept is a synthetic design concept that can be used for next-step synthetic planning and execution. PSP provides a tool to design new materials platforms by focusing on chemistry and topology. The growing importance of small-molecule gas storage and separation has led to the development of small-pore materials using the uniquely suited PSP strategy. The partitioned-acs (pacs) platform is the best embodiment of the PSP concept and has resulted in a large family of chemically robust materials with controllable pore metrics and suitable functionalities.
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Fahui Xiang et al.
Summary: Stimuli-responsive proton-conducting metal-organic frameworks (MOFs) have attracted attention due to their potential applications. This Perspective highlights the current progress in the rational design and fabrication of switchable proton-conducting MOFs, discussing the dynamic structural changes of proton transfer pathways and the role of trigger molecules. Challenges and new research opportunities for further development are also discussed.
Review
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Soheila Sanati et al.
Summary: This review focuses on the use of MOF-derived bimetallic materials in supercapacitors, highlighting their advantages including tunable electrochemical activity, high charge capacity, and improved electrical conductivity. The challenges and perspectives in this research area are also discussed.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2021)
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Chemistry, Inorganic & Nuclear
Ehsan Binaeian et al.
Summary: This article discusses the removal of ammonia, hydrogen sulfide, sulfur dioxide, and volatile organic compounds, introducing the design and synthesis achievements of metal-organic frameworks (MOFs) as adsorbents.
COORDINATION CHEMISTRY REVIEWS
(2021)
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Cong Li et al.
Summary: Improving discharge-charge reversibility by enhancing structural stability through in situ growth of MOF-derived V2O3 on carbon cloth has demonstrated high capacity retention and cycling stability. The stable cathode structure and oxygen vacancy defects play a crucial role in achieving high discharge specific capacity.
Review
Chemistry, Physical
Shyam Chand Pal et al.
Summary: Solid-state proton-conducting materials, such as hydrogen-bonded organic frameworks (HOFs), are essential in various electrochemical devices like fuel cells. HOFs with well-defined H-bonded networks exhibit high stability with permanent microporosity, making them versatile platforms for solid-state proton conductors showing high conductivity potential. The development of HOFs as proton conductors, along with the considerations of early reports on proton-conducting systems and alternative terminologies, is discussed in depth in this review, with a focus on the design principles and critical features for realizing efficient conduction properties.
ACS ENERGY LETTERS
(2021)
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Yu-Chang Wang et al.
Summary: This article focuses on the research of metal-organic frameworks (MOFs) and their composites as photocatalysts, highlighting their structural strategies, photoelectron trajectories, and structure-function relationship. The potential of these photocatalysts in pollutants degradation, water splitting for H-2 generation, and CO2 reduction is emphasized for future high-efficiency catalyst design.
CHEMICAL ENGINEERING JOURNAL
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Summary: The study developed a metal organic framework-based fluorescent sensor for effective detection of Al(III) with a low detection limit of 17.5 ppb, even in the presence of other metal ions. The research also demonstrated a method of real-time naked eye observation using MOF filter paper tests.
CHEMISTRY-A EUROPEAN JOURNAL
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Chunfei Wang et al.
Summary: Coordination-based molecular nanomaterials with well-defined chemical structures, high synthetic reproducibility, and diverse functionalities bridge the gap between small molecules and conventional nanomaterials. They have shown great potential in biomedically relevant applications such as biosensing, bioimaging, and therapy.
COORDINATION CHEMISTRY REVIEWS
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Chemistry, Physical
Rupam Sahoo et al.
Summary: COFs are a promising class of solid-state proton-conducting materials with high structural tunability and excellent properties, making them versatile platforms for electrochemical devices. This review discusses the strategies, structure-function relationships, challenges, and future prospects of COFs as proton conductors in detail.
ADVANCED ENERGY MATERIALS
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T. Paul et al.
Summary: In this paper, DRT functions are numerically calculated for different systems with impedance data, and the quality of impedance data is checked using Kramers-Kronig relations. The DRTs are calculated using Tikhonov regularization method and the physical significance of peaks are discussed through peak fitting program.
SCIENTIFIC REPORTS
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Prakas Samanta et al.
Summary: Rechargeable aqueous Zn-ion batteries have drawn attention for their low cost and environmental friendliness. The performance of these batteries can be enhanced by involving both cationic and anionic redox conversion mechanisms simultaneously.
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Rupam Sahoo et al.
Summary: Gas separation processes have a significant impact on various sectors globally. The removal of C-2 hydrocarbons from natural gas is a crucial step, with MOFs offering promise for such separations. Challenges and future prospects in this area are discussed in detail for further development.
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