Journal
CHEMICAL COMMUNICATIONS
Volume 51, Issue 77, Pages 14458-14461Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c5cc05072c
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Funding
- European Community (FP7) [228862]
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Crystallisation of a mixed-metal form of the porous framework UiO-66 in which Zr is partially replaced by Ce produces a liganddefective material, that contains some Ce(III) as well as a majority of Ce(IV). Infrared spectroscopy shows enhanced binding of methanol in the substituted material that leads to catalytic decomposition of the alcohol, which may be due to a combination of defects and redox activity.
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