Journal
ACTA MATERIALIA
Volume 257, Issue -, Pages -Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.actamat.2023.119145
Keywords
Stacking-fault tetrahedron; Frank loop; Palladium; Irradiation; Molecular dynamics simulations
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Stacking-fault tetrahedron (SFT) is a three-dimensional vacancy defect that can seriously degrade the mechanical properties of quenched, deformed or irradiated face-centered cubic (FCC) metals. It is generally believed that high stacking fault energy (SFE) is unfavorable for the formation of SFTs. However, this study reveals a new mechanism for the formation of SFTs in Pd with extremely high SFE, where vacancy clusters rearrange directionally to form SFTs due to the ambient stress deviations and compressive stress fields induced by interstitial Frank loops. Continuous hydrogen implantation promotes the growth of the complex, while thermal effects can cause it to disappear.
Stacking-fault tetrahedron (SFT) is one kind of typical three-dimensional vacancy defect in quenched, deformed or irradiated face-centered cubic (FCC) metals, which can seriously degrade the mechanical properties of materials. It's generally believed that high stacking fault energy (SFE) is unfavorable for the formation of SFTs. Here, we report the first in-situ investigation of irradiation-induced formation of novel Frank loop-SFT complexes in Pd with extremely high SFE. Our findings reveal a new mechanism that vacancy clusters rearrange directionally to form SFTs due to the ambient stress deviations and compressive stress fields induced by interstitial Frank loops. Continuous hydrogen implantation will lead to a synergistic growth of the complex, while direct interaction between the Frank loop and SFT under thermal effect can cause the complex to disappear. These results uncover a unique formation mechanism for SFT and provide a new perspective for understanding nanodefects in high SFE metals.
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