Halide Tunablility Leads to Enhanced Biomechanical Energy Harvesting in Lead-Free Cs2SnX6-PVDF Composites

Article Energy & Fuels

High-Performance Flexible Piezo-Tribo Hybrid Nanogenerator Based on MoS2@ZnO-Assisted β-Phase-Stabilized Poly(Vinylidene Fluoride) Nanocomposite

Suparna Ojha et al.

Summary: The combination of piezoelectric and triboelectric effects in a fabricated hybrid nanogenerator shows excellent performance in energy harvesting from mechanical and biological movements, with potential applications in biomedical field.

ENERGY TECHNOLOGY (2023)

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Article Chemistry, Inorganic & Nuclear

Solution-processed light-induced multilevel non-volatile wearable memory device based on CsPb2Br5 perovskite

Tufan Paul et al.

Summary: Despite recent advancements, the quest for building materials with low power consumption in memory devices continues. This study explores the use of halide perovskites as a switching layer in memory devices, specifically focusing on the CsPb2Br5 film. The device exhibits pronounced bipolar resistive switching and shows promising features such as uniform switching, high endurance, and long retention time. Additionally, the device maintains its performance even under bending conditions.

DALTON TRANSACTIONS (2022)

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Article Nanoscience & Nanotechnology

Temperature-dependent dielectric properties of CsPb2Br5: a 2D inorganic halide perovskite

Aditi Sahoo et al.

Summary: 2D CsPb2Br5 synthesized through chemical precipitation method exhibits high dielectric constant and low dielectric loss, showing great potential in energy harvesting and storage devices.

NANOTECHNOLOGY (2022)

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Article Chemistry, Physical

Revisiting of 8-PVDF nanoparticles via phase separation with giant piezoelectric response for the realization of self-powered biomedical sensors

Hari Krishna Mishra et al.

Summary: Piezo-, pyro-, ferro-electricity in carbon-fluoro polymers such as poly(vinylidene fluoride) (PVDF) and its copolymers are gaining technological interest in self-powered flexible electronics. Achieving nanostructures of PVDF with preferred electroactive phase and enhanced piezoelectric coefficient is still a challenge. This study introduces a nanoprecipitation technique to machinate PVDF nanoparticles with predominant piezoelectric delta phase using the bi-solvent phase separation technique. The resulting delta-PVDF nanoparticles exhibit excellent piezoelectric properties and potential applications in self-power sensors and actuators.

NANO ENERGY (2022)

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Article Chemistry, Multidisciplinary

Stretchable, Breathable, and Stable Lead-Free Perovskite/Polymer Nanofiber Composite for Hybrid Triboelectric and Piezoelectric Energy Harvesting

Feng Jiang et al.

Summary: This study presents a lead-free perovskite-based nanofiber composite (LPPS-NFC) as a stretchable, breathable, and stable material for energy harvesting. The LPPS-NFC demonstrates excellent electrical output and mechanical properties, making it a promising material for wearable devices that convert mechanical energy into electrical power.

ADVANCED MATERIALS (2022)

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Article Chemistry, Multidisciplinary

Superstable and Intrinsically Self-Healing Fibrous Membrane with Bionic Confined Protective Structure for Breathable Electronic Skin

Miaomiao Zhu et al.

Summary: A novel interface protective strategy is reported in this article to develop intrinsically self-healing fibrous membranes with a bionic confined structure, which are further assembled into an all-fiber structured electronic skin. The electronic skin is multifunctional with self-powering, self-healing, breathability, stretchability, and thermochromism functionalities.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2022)

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Article Multidisciplinary Sciences

A method for quantitatively separating the piezoelectric component from the as-received Piezoelectric signal

Chaojie Chen et al.

Summary: A simple and effective method is proposed to quantitatively identify and extract the piezoelectric charge from hybrid signals, elucidating the true performance of piezoelectric devices.

NATURE COMMUNICATIONS (2022)

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Article Materials Science, Multidisciplinary

All-inorganic halide perovskite tuned robust mechanical-energy harvester: Self driven posture monitor and power source for portable electronics

Suvankar Mondal et al.

Summary: Scavenging electric power from biomechanical movements and vibrations using piezoelectric nanogenerators has become an accessible energy alternative. The incorporation of caesium lead chloride in polyvinylidene fluoride films enhances the piezoelectric properties. The fabricated PNGs demonstrate high sensitivity and flexibility, making them suitable for wearable sensors and portable devices.

APPLIED MATERIALS TODAY (2022)

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Article Chemistry, Physical

High Ionic Conduction and Polarity-Induced Piezoresponse in Layered Bimetallic Rb4Ag2BiBr9 Single Crystals

Manoj Singh et al.

Summary: The emergence of lead-free metal-halide perovskites in modern-day energy research is primarily due to their competent semiconducting and optoelectronic properties, as well as their nontoxicity and improved stability in ambient operating conditions. In this article, the authors report on the single-crystal growth of a bimetallic two-dimensional layered Rb4Ag2BiBr9 and explore its dielectric, piezoelectric, and ferroelectric properties. They investigate the dielectric attributes by studying the temperature-dependent complex impedance, complex electric modulus, and AC conductivity, and analyze the ion transport and relaxation mechanisms in Rb4Ag2BiBr9. The authors also demonstrate the thermal and ambient stability of the material, as well as its piezoelectric and ferroelectric properties.

JOURNAL OF PHYSICAL CHEMISTRY C (2022)

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Article Materials Science, Multidisciplinary

Onset of vacancy-mediated high activation energy leads to large ionic conductivity in two-dimensional layered Cs2PbI2Cl2 Ruddlesden-Popper halide perovskite

Nisha Hiralal Makani et al.

Summary: In this study, the dielectric properties of a two-dimensional layered perovskite Cs2PbI2Cl2 were investigated using various experimental techniques and theoretical models. It was found that the ionic conductivity of the material increases abruptly at a critical temperature, which is attributed to enhanced ionic conduction mediated by anionic vacancies.

PHYSICAL REVIEW MATERIALS (2022)

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Article Chemistry, Analytical

Photoelectrocatalytic CO2 reduction using stable lead-free bimetallic CsAgBr2 halide perovskite nanocrystals

Nisha Hiralal Makani et al.

Summary: In this study, highly stable lead-free CsAgBr2 perovskite nanocrystals (PNC) were fabricated at room temperature without the involvement of any organic ligand. The synthesized PNC showed good structural stability, air stability for up to six months, and thermal stability up to 200 degrees C. Furthermore, the PNC exhibited superior photoelectrocatalytic CO2 reduction performance.

JOURNAL OF ELECTROANALYTICAL CHEMISTRY (2022)

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Article Chemistry, Multidisciplinary

Lead-Free Perovskite Cs3Bi2I9-Derived Electroactive PVDF Composite-Based Piezoelectric Nanogenerators for Physiological Signal Monitoring and Piezo-Phototronic-Aided Strained Modulated Photodetectors

Bidya Mondal et al.

Summary: Lead-free perovskite materials have gained significant attention in photovoltaic and optoelectronic applications due to their low toxicity and superior optical properties. This study introduces a stable lead-free Cs3Bi2I9-PVDF composite and demonstrates its potential as a material for piezoelectric nanogenerators and photodetectors.

LANGMUIR (2022)

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Article Chemistry, Physical

High piezoresponse in low-dimensional inorganic halide perovskite for mechanical energy harvesting

Aditi Sahoo et al.

Summary: The low-dimensional all-inorganic halide perovskite material CsPb2Br5 demonstrates piezoelectric and ferroelectric behavior at room temperature and shows great potential as a functional material for energy harvesting devices. The composite of CsPb2Br5 microplates with PVDF exhibits excellent energy harvesting performance in piezoelectric-based mechanical energy harvesters.

SUSTAINABLE ENERGY & FUELS (2022)

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Article Chemistry, Physical

The mechanism of a PVDF/CsPbBr3 perovskite composite fiber as a self-polarization piezoelectric nanogenerator with ultra-high output voltage

You Xue et al.

Summary: The self-polarization effect in PVDF/CsPbBr3 composite fibers is studied, which demonstrates outstanding voltage output under self-polarization conditions. The mechanism of self-polarization is revealed by analyzing the interfacial charge and electric field. The research also validates the practical applicability of PVDF/CsPbBr3-PENG in harvesting energy from human finger taps and tests its stability.

JOURNAL OF MATERIALS CHEMISTRY A (2022)

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Article Chemistry, Multidisciplinary

Tin-based halide perovskite materials: properties and applications

Mahdi Malekshahi Byranvand et al.

Summary: Organic-inorganic hybrid halide perovskite materials have attracted significant research interest, particularly in the field of photovoltaics. However, the toxicity of lead in these materials limits their applications, prompting the search for alternatives. Tin-based perovskites have shown the highest potential as substitutes, but challenges in stability, safety, and commercialization still need to be addressed.

CHEMICAL SCIENCE (2022)

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Article Chemistry, Physical

Lead-free Cs2SnX6 (X = Cl, Br, I) nanocrystals in mesoporous SiO2 with more stable emission from VIS to NIR light

Ziyu Pan et al.

Summary: Lead-free double-perovskite Cs2SnX6 nanocrystals were successfully synthesized and loaded into SiO2, demonstrating stability in both solution and air. These composite nanoparticles show potential medical applications, such as photothermal and photodynamic therapies for cancers.

CHEMICAL PHYSICS LETTERS (2021)

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Article Chemistry, Physical

How Far Are We from Achieving Self-Powered Flexible Health Monitoring Systems: An Energy Perspective

Hui Yu et al.

Summary: The review investigates whether current flexible energy devices can meet the energy demand of wireless flexible sensor systems in long-term health monitoring applications. It estimates the total energy demand of typical sensor systems and discusses the design of the energy supply architecture. Health monitoring protocols that could be realized with self-powered system designs are suggested, and core challenges for further development of the technologies for practical applications are identified.

ADVANCED ENERGY MATERIALS (2021)

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Article Materials Science, Multidisciplinary

Cube shaped FAPbBr3 for piezoelectric energy harvesting devices

Tufan Paul et al.

Summary: Organic-inorganic halide perovskites are a relatively new class of compounds with potential for energy harvesting. Prepared FAPbBr(3) cubes via solution process showed significant output performance in energy harvesting, demonstrating long cycle stability and durability.

MATERIALS LETTERS (2021)

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Review Chemistry, Physical

Recent developments in self-powered smart chemical sensors for wearable electronics

Aaryashree et al.

Summary: The future of electronics technology will be primarily based on wearable sensing systems, with wearable electronic sensors that do not require external power sources being crucial for portable and mobile applications. This review article presents the recent progress of wearable self-powered smart chemical sensors systems, as well as an overview of various energy conversion and storage technologies for self-powered devices.

NANO RESEARCH (2021)

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Article Chemistry, Multidisciplinary

Making use of nanoenergy from human - Nanogenerator and self-powered sensor enabled sustainable wireless IoT sensory systems

Minglu Zhu et al.

Summary: This review discusses the applications of wearable and implantable piezoelectric nanogenerator (PENG) and triboelectric nanogenerator (TENG) in digitizing the human body, exploring different mechanical stimuli and materials. It also explores the potential of self-powered physical sensors and the enhancement of energy generation and sensing performance through hybrid systems.

NANO TODAY (2021)

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Article Chemistry, Physical

Paper-Based Stable Broad Band Optical Detector Made from Mixed Cation Organic Perovskite Halides

Avisek Maity et al.

Summary: The paper reports a paper-based photodetector made from mixed cation organic perovskite halide MA(1-x)FA(x)PbI(3) with high photogain and broad band response. It shows peak responsivity of 0.27 A/W at a wavelength of around 775 nm and remains above 0.1 A/W for a wide optical wavelength range. The detector has low dark current, low power consumption, and is suitable for applications requiring flexible and disposable detectors.

JOURNAL OF PHYSICAL CHEMISTRY C (2021)

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Article Materials Science, Multidisciplinary

Universal sensing of ammonia gas by family of lead halide perovskites based on paper sensors: Experiment and molecular dynamics

Avisek Maity et al.

Summary: This paper demonstrates the fabrication of high sensitivity and high selectivity room temperature ammonia gas sensors using lead halide perovskites. These sensors can sensitively detect NH3 gas through simple color and resistance changes, and operate below ppm levels with low power consumption.

MATERIALS RESEARCH BULLETIN (2021)

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Article Chemistry, Physical

Electrochemical Performance of 3D Network CsPbBr3 Perovskite Anodes for Li-Ion Batteries: Experimental Venture with Theoretical Expedition

Tufan Paul et al.

Summary: The study presents the usage perspective of CsPbBr3 as an active anode material in Li-ion batteries, demonstrating its good performance and stability through experimental and theoretical investigations.

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Highly radiation resistant room temperature organic perovskite halide (FAPbI3) crystal for direct detection of gamma-ray photons down to nano curie activity

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Summary: A simple room temperature gamma-ray detector made from highly textured crystals of organic perovskite halide formamidium lead iodide (FAPI) was reported in this study, with electrical readout using resistance changes similar to optical detectors. The detector can detect presence of gamma-rays in a wide energy range from 100 to 1250 keV with noise-limited sensitivity capable of detecting activity down to 50 nCi, and has a reasonable mu tau approximate to 5.2 x 10(-3)cm(2)V(-1) gamma-ray, making it suitable for applications requiring long exposure. Additionally, a proof of concept for wearable, low-cost, portable solid state gamma ray detectors using paper electronics based halide perovskites has been established.

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Autonomous self-repair in piezoelectric molecular crystals

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Halide Tunablility Leads to Enhanced Biomechanical Energy Harvesting in Lead-Free Cs2SnX6-PVDF Composites

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