Journal
CHEMICAL COMMUNICATIONS
Volume 51, Issue 47, Pages 9706-9709Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c5cc03143e
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Funding
- National Basic Research Program of China [2013CB632405]
- NSF of China [21425309, 21173043]
- State Key Laboratory of NBC Protection for Civilian [SKLNBC2013-04 K]
- Specialized Research Fund for the Doctoral Program of Higher Education [20133514110003]
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Incorporation of aromatic motifs into the nanosized shells of hollow carbon nitride nanospheres has been reported to develop functional photosynthetic structures for solar energy application. This modification results in an extended pi-conjugation system, red-shift of the optical absorption, and an improved charge separation in the shell, while still retaining the unique hollow polymeric nanoarchitectures. This strategy enables the tuning of the semiconductor properties of the shell substance in the hollow carbon nitride nanostructures to generate the redox species to enhance photocatalytic activity for hydrogen evolution using visible light.
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