3.9 Article

Photoinduced excited-state dynamics in Co-doped BaFe2As2 superconducting films

Journal

MRS ADVANCES
Volume 8, Issue 5, Pages 161-166

Publisher

SPRINGER HEIDELBERG
DOI: 10.1557/s43580-023-00513-5

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The Co-doped BaFe2As2 superconducting films exhibit complex nonlinear optical dynamics and structural transformation over a wide range of temperatures. The angle-resolved light scattering conoscopy reveals the temperature-dependent structural transformation of optimally doped BaFe2As2. Photoinduced excited states dynamics demonstrate the instantaneous formation of nonequilibrium quasiparticles, followed by multi-step thermalization within several picoseconds. These transient processes show noticeable temperature dependence below the superconducting transition point Tc, where they correlate with the surface morphology.
The nonlinear optical dynamics and structural transformation of Co-doped BaFe2As2 superconducting films demonstrate complex behavior within a broad range of temperatures. The angle-resolved light scattering conoscopy reveals the temperature-dependent structural transformation of the optimally doped BaFe2As2. Photoinduced excited states dynamics demonstrate the instantaneous formation of the nonequilibrium state of quasiparticles with its subsequent multi-step thermalization within several picoseconds. These transient processes show noticeable temperature dependence below superconducting transition point T-c, where photoinduced dynamics correlate with the surface morphology.

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