Journal
ACS APPLIED ENERGY MATERIALS
Volume 6, Issue 4, Pages 2257-2264Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acsaem.2c03416
Keywords
perovskite; single crystals; solar cells; aging; enhancement
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Single-crystal perovskite solar cells exhibit spontaneous efficiency enhancement due to the slow release of trapped solvent in the perovskite thin films. Heat treatment of the films at 40 degrees C can accelerate solvent release and further improve the performance of the solar cells. This study provides a theoretical basis for advancing single-crystal perovskite solar cells.
Perovskite solar cells show spontaneous efficiency enhancement (SEE), i.e., their efficiency improves with time over a few days. Many mechanisms have been proposed for explaining such behavior in polycrystalline perovskite solar cells. However, such studies have not been performed on single-crystal perovskite solar cells. Here, we report our observation of slow (similar to 20 days) SEE in methylammonium lead iodide single-crystal perovskite solar cells. We found that the SEE is due to the slow escape of solvent trapped by the perovskite single-crystal thin films. We show that this process can be substantially accelerated by heat treatment of cells at 40 degrees C. This work provides a ground for fast-tracking the progress of single-crystal perovskite solar cells.
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