Journal
CHEMCATCHEM
Volume 7, Issue 7, Pages 1048-1057Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cctc.201500032
Keywords
chemoselectivity; encapsulation; heterogeneous catalysis; hydrogen spillover; model catalyst
Categories
Funding
- Basic Science Research Program through the National Research Foundation of Korea (NRF) [NRF-2011-0011392]
- Advanced Biomass R&D Center (ABC) of Global Frontier Project - Ministry of Education, Science and Technology [ABC-2011-0031356]
- Korea CCS R&D Center (KCRC) - Korea government (Ministry of Science, ICT & Future Planning) [NRF-2014M1A8A1049256]
- National Research Foundation of Korea [2010-0029728, 2014M1A8A1049256, 2011-0011392, 10Z20130011056] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
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Hydrogen spillover has been one of the most debated concepts in the field of heterogeneous catalysis due to limited ways of studying it. The main controversies in hydrogen spillover, especially from the viewpoint of its catalytic functions, can be mainly attributed to the absence of well-defined model catalysts that can provide direct proof of the catalytic functions of hydrogen spillover. In this article, we will provide an overview of the recent progress made with encapsulated metal catalysts, which can act as an ideal model catalyst for proving the existence and catalytic functions of hydrogen spillover. We will also demonstrate unique opportunities of using the encapsulated metal catalysts for designing advanced hydroprocessing catalysts with enhanced activity, distinct chemoselectivity, and increased catalyst durability.
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