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Physics, Condensed Matter
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Summary: We report the discovery and investigation of superconductivity in Mo4Ga20As, which crystallizes in the I4/m space group with lattice parameters a = 12.86352 angstrom and c = 5.30031 angstrom. It exhibits type-II superconductivity with a critical temperature of 5.6 K and estimated upper and lower critical fields of 2.78 T and 22.0 mT, respectively. The electron-phonon coupling in Mo4Ga20As is likely stronger than the BCS weak-coupling limit, and first-principles calculations reveal the dominance of Mo-4d and Ga-4p orbitals in the Fermi level.
JOURNAL OF PHYSICS-CONDENSED MATTER
(2023)
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Physics, Multidisciplinary
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Summary: We investigated the crystal structure and electronic properties of the heavy fermion superconductor UTe2 at high pressure using X-ray diffraction and electrical resistivity experiments. The X-ray diffraction measurements reveal that the unit cell has anisotropic linear compressibility up to 3.5 GPa, and a pressure-induced structural phase transition occurs above 3.5-4 GPa at room temperature. The molar volume decreases abruptly, while the distance between neighboring U atoms increases, indicating a transition from heavy electronic states to weakly correlated ones. Surprisingly, a new superconducting phase with a relatively low upper-critical field was detected at pressures above 7 GPa.
JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN
(2023)
Review
Physics, Applied
Kazumasa Iida et al.
Summary: Since the discovery of Fe-based superconductors, efforts have been made to grow single crystals and epitaxial thin films of them for both fundamental studies and applied research. Remarkably, most Fe-based superconductors have been successfully realized in the form of epitaxial thin films. However, due to various challenges, some compounds could only be obtained as single crystals. In recent years, these issues have been solved, and those compounds have been successfully fabricated as epitaxial thin films, allowing for easier evaluation of their application potential through transport critical current measurements.
SUPERCONDUCTOR SCIENCE & TECHNOLOGY
(2023)
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Bai Yang Wang et al.
Summary: The search for superconductivity in infinite-layer nickelates, inspired by the cuprates, has encountered debates regarding the impact of varying rare-earth elements on these materials. In this study, we observe significant differences in the magnitude and anisotropy of the superconducting upper critical field across different rare-earth nickelates, namely La-, Pr-, and Nd-nickelates. These differences originate from the 4f electron characteristics of the rare-earth ions in the lattice, with La3+ being absent, Pr3+ being nonmagnetic, and Nd3+ being magnetic. The unique magnetoresistance found in Nd-nickelates can be attributed to the magnetic contribution of Nd3+ 4f moments. The robust and tunable superconductivity exhibited by these materials holds promise for future high-field applications.
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Chemistry, Physical
Nikolai D. Zhigadlo et al.
Summary: We present a study on the electronic properties of LaFeAsO single crystals co-substituted with Sm and P, both in normal and superconducting states. The appearance of superconductivity is believed to be caused by the inner chemical pressure induced by the smaller-size isovalent substituents. The results demonstrate the potential of co-substitution as a method to induce superconductivity in the 1111 family, opening up new possibilities for the design and creation of superconductors through chemical manipulation.
JOURNAL OF ALLOYS AND COMPOUNDS
(2023)
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T. Shang et al.
Summary: We have investigated the NiBi3 single crystals using electrical-resistivity, magnetization, and muon-spin rotation and relaxation (mu SR) measurements. The single crystal of NiBi3 exhibits bulk superconductivity with T-c around 4.1 K and weakly anisotropic superconductivity. The temperature evolution of the superfluid density reveals a fully gapped superconductivity in NiBi3, with shared superconducting gap Lambda(0) = 2.1k(B)T(c) and magnetic penetration depths lambda(0) = 223 and 210 nm for H parallel to b and H perpendicular to b, respectively. The absence of spontaneous fields and any type of magnetic ordering in NiBi3 single crystals suggests it behaves as a conventional s-type superconductor.
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Materials Science, Multidisciplinary
He Zhang et al.
Summary: In this work, the superconductivity observed in PbS by pressure engineering is reported. PbS undergoes electronic phase transitions upon compression, and superconductivity occurs above 23.9 GPa in the high-pressure CsCl-type cubic phase. Further compression suppresses the superconductivity while the Tc is reduced. It is noted that PbS is one of the few binary metal sulfide superconductors with a Tc above 10 K, and it exhibits unexpected multiband behavior, benefiting the study of pressure-induced superconductivity.
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Multidisciplinary Sciences
Jie Yuan et al.
Summary: The research uncovers the precise quantitative scaling laws among the superconducting transition temperature, the linear-in-T scattering coefficient, and the doping level in electron-doped copper oxide La2-xCexCuO4, suggesting a common mechanism of the strange-metal behavior and unconventional superconductivity in these systems.
Article
Chemistry, Physical
Grace A. Pan et al.
Summary: This study reports the synthesis of Nd6Ni5O12, a new type of superconducting nickelate material that achieves optimal cuprate-like electron filling without the need for chemical doping. The material exhibits a superconducting transition around 13K and displays behavior intermediate between cuprate-like and infinite-layer nickelate-like behavior. This indicates that square-planar nickelates are a new family of superconductors that can be tuned through both doping and dimensionality.
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S. W. Zeng et al.
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Summary: This article summarizes recent research on the many-body electronic structure of layered rare-earth nickelates, comparing them to high-temperature superconducting copper-oxide compounds. It focuses on understanding how the interacting physics can be estimated and downfolded into a low energy theory to describe relevant degrees of freedom.
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Summary: This study investigates the gap structure and anisotropy of RbCa2(Fe1-xNix)(4)As4F2 single crystals by combining directional point-contact Andreev-reflection spectroscopy and coplanar waveguide resonator measurements. The results show that the compound has two gaps with d-wave-like nodal structures, which persist upon Ni doping, and that its anisotropy is in good agreement with the d-d model.
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(2022)
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Chemistry, Physical
Xin Gui et al.
Summary: This research reports the discovery of superconductivity below 5.2K in LaIr3Ga2, a previously unreported material based on stacked Kagome planes. The superconductor is characterized experimentally, and calculations reveal that the electronic structure is significantly influenced by spin-orbit coupling. This material is considered important for investigating the coupling between topological physics and superconductivity.
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Physics, Applied
Dong Li et al.
Summary: The magneto-transport properties of a series of single-crystal films of intercalated iron-selenide superconductor (Li,Fe)OHFeSe were systematically measured under c-direction fields up to 33 T. A new vortex-phase diagram was established for the weakly-disordered high-T (c) (Li,Fe)OHFeSe, showing an emergent dissipative vortex phase intermediate between the common vortex glass and liquid phases.
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Ritu Gupta et al.
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NPJ QUANTUM MATERIALS
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Sam Mugiraneza et al.
Summary: Magnetic susceptibility measurements are crucial in assessing the magnetic nature of newly discovered materials. While collecting high quality data has become more accessible, the analysis of the data remains a challenge for newcomers. This guide focuses on materials exhibiting Curie-Weiss paramagnetism and provides a basic understanding of magnetic susceptibility data analysis and interpretation.
COMMUNICATIONS PHYSICS
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Jeong Min Park et al.
Summary: Superconductivity has been observed in magic-angle twisted four-layer and five-layer graphene systems, expanding the family of moire superconductors. The distinction between the twisted bilayer graphene and other members of the family is related to the movement of electrons between layers in a magnetic field. This discovery provides new insights for the design of superconducting materials platforms.
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Physics, Multidisciplinary
Jennifer Fowlie et al.
Summary: Muon spin rotation/relaxation studies have revealed the coexistence of intrinsic magnetic ground state and superconductivity in superconducting infinite-layer nickelates, regardless of rare earth ion or doping. This magnetism, likely to be antiferromagnetic and short-range ordered, is qualitatively distinct from doped cuprates and resembles that of some iron pnictides and heavy fermion compounds.
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Physics, Multidisciplinary
Matteo Rossi et al.
Summary: A charge ordering state has been observed in nickelate superconductors, which is distinct from other observed ordered states. The results suggest that strong electronic correlations may be responsible for this ordered state, and the interplay between charge order, antiferromagnetic fluctuations, and superconductivity is an important topic in nickel-based superconductors.
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G. Krieger et al.
PHYSICAL REVIEW LETTERS
(2022)
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Andreas Kreisel et al.
Summary: The study investigated the superconducting properties of infinite-layer nickelates, revealing a superconducting instability transition driven by strong fluctuations in the dz2 orbital states. The properties of the superconducting condensates were discussed based on experiments probing the detailed superconducting gap structure.
PHYSICAL REVIEW LETTERS
(2022)
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N. N. Wang et al.
Summary: The successful synthesis of high-quality Pr0.82Sr0.18NiO2 thin films with a superconducting onset temperature Tc(onset) of approximately 17 K and the observation of Tc(onset) increasing to approximately 31 K under a pressure of 12.1 GPa suggest that there is still potential to further enhance the Tc of infinite-layer nickelates through higher pressures or strain engineering in heterostructure films.
NATURE COMMUNICATIONS
(2022)
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Multidisciplinary Sciences
Casey K. W. Leung et al.
Summary: High-entropy alloys form through the random arrangement of chemical elements and some of them can enter a superconducting state. We have conducted magnetic susceptibility measurements on a superconducting high-entropy alloy and found that it behaves as a single-band isotropic s-wave superconductor in the dirty limit.
SCIENTIFIC REPORTS
(2022)
Article
Chemistry, Physical
Charles C. Tam et al.
Summary: CDWs were observed in infinite-layer nickelates films with Ni L-3 resonant X-ray scattering, forming at a specific commensurate wavevector related to Nd 5d-Ni 3d orbitals, and disappearing upon 20% Sr doping.
Article
Materials Science, Multidisciplinary
C. L. Zhang et al.
Summary: Studies on polyhydrides are attracting growing attentions recently due to their potential high temperature superconductivity. Here, the authors report the discovery of superconductivity in hafnium polyhydrides at high pressures, with the superconducting phase identified as C2/ m-HfH14 and a high Tc observed. This is the first 5d transition metal polyhydride superconductor with Tc above the liquid nitrogen temperature.
MATERIALS TODAY PHYSICS
(2022)
Article
Materials Science, Multidisciplinary
T. Y. Xie et al.
Summary: This study presents a microscopic theory for the electronic structure of nickelates based on a fundamental model, revealing the dominance of Mottness and Hundness in the appearance of weak insulator phases and superconducting phases in different hole-doped regimes. It also demonstrates the unique orbital-selective doping and provides a unified understanding of the superconducting phase diagram in hole-doped infinite-layer nickelates, which is distinct from other types of superconductors.
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Materials Science, Multidisciplinary
Jonathan Karp et al.
Summary: The study compares the properties of nickelate and cuprate compounds, finding that they exhibit antiferromagnetic and superconducting behavior, respectively, under stoichiometric conditions. The results also suggest that nickelate superconductivity is similar to cuprate superconductivity but requires a higher level of doping.
Article
Materials Science, Multidisciplinary
Chen Lu et al.
Summary: This study investigates the pairing mechanism and symmetry in newly synthesized strontium doped RNiO2 superconductors. The results reveal that the leading pairing symmetry is the intraorbital dx2-y2-wave singlet pairing, similar to cuprates. However, there are two important differences between the physical properties of the two families, which can be verified by angle-resolved photoemission spectrum.
Article
Physics, Multidisciplinary
Bai Yang Wang et al.
Summary: Recent studies have observed superconductivity in nickelates, prompting the proposal of various candidate models to understand this phenomenon. By using magnetotransport measurements, researchers were able to probe the superconducting anisotropy in nickelates and found surprising isotropy in the upper critical field despite the layered crystal structure. This suggests that the superconductivity in nickelates is Pauli-limited, unlike traditional layered oxides.
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Berit H. Goodge et al.
Summary: The recent discovery of superconductivity in Nd0.8Sr0.2NiO2 has led to questions about the underlying electronic structure hierarchy. By using locally resolved electron energy-loss spectroscopy, the Mott-Hubbard character of Nd1-xSrxNiO2 was directly probed, revealing evidence of a multiband electronic structure in the superconducting infinite-layer nickelates.
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA
(2021)
Article
Physics, Applied
D. Y. Yan et al.
Summary: We report the synthesis and physical properties of single crystals of TaC, a proposed topological superconductor candidate with a critical temperature of 10.3 K. TaC is a bulk superconductor described by s-wave BCS theory with a single gap, and exhibits linear temperature dependence in the upper critical field (H-c2), distinguishing it from most conventional superconductors. This suggests TaC as a new candidate for further research in topological superconductors.
SUPERCONDUCTOR SCIENCE & TECHNOLOGY
(2021)
Article
Chemistry, Physical
I. Leonov
Summary: In this study, the effects of electron-electron interactions and Sr doping on the electronic structure of (Nd,Sr)NiO2 were investigated using the DFT+DMFT approach. It was found that Sr doping led to a Lifshitz transition, causing a reconstruction of magnetic correlations and changes in electronic properties. The results suggest that in-plane strain plays a crucial role in adjusting the band structure of (Nd,Sr)NiO2, influencing both its electronic structure and magnetic correlations.
JOURNAL OF ALLOYS AND COMPOUNDS
(2021)
Article
Physics, Multidisciplinary
S. Kasahara et al.
Summary: Investigating the superconducting order parameter in FeSe single crystal at high magnetic fields, thermodynamic evidence for a distinct superconducting phase was provided by heat capacity and magnetic torque measurements. Spectroscopic-imaging scanning tunneling microscopy revealed the disappearance of superconducting order parameter at the surface upon entering the high-field phase, demonstrating a pinned planar node perpendicular to the magnetic field.
PHYSICAL REVIEW LETTERS
(2021)
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Physics, Multidisciplinary
J. Q. Lin et al.
Summary: The discovery that d(9-delta) nickelates can host a large superexchange has sparked diverse theoretical perspectives on the fundamental physics of this class of materials. The findings suggest that layered nickelates could represent an intermediate case between infinite-layer nickelates and cuprates, providing a pathway for testing the relevance of superexchange to nickelate superconductivity.
PHYSICAL REVIEW LETTERS
(2021)
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Physics, Multidisciplinary
Chang-Jong Kang et al.
Summary: The study reveals the optical properties of the infinite-layer La1-xSrxNiO2 in its normal state, showing a correlated metal state with unique behaviors compared to density functional theory, such as decreasing integrated optical spectral weight with doping and increasing temperature. The effective crystal field splitting is found to be dynamic, leading to the formation of a Hund's metallic state with dynamic orbital fluctuations at intermediate energies.
PHYSICAL REVIEW LETTERS
(2021)
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T. Takenaka et al.
Summary: Metal-organic frameworks (MOFs) provide a tunable platform for exploring new states of matter through self-assemblies of metal ions and organic ligands. The discovery of superconductivity in the π - d conjugated 2D MOF [Cu3(C6S6)](n) (Cu-BHT) with a critical temperature Tc of 0.25 kelvin raises questions about the nature of electron pairing. The unconventional superconductivity in Cu-BHT is believed to originate from electron correlations related to spin fluctuations of the kagome lattice, with an extremely low superfluid density.
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Materials Science, Multidisciplinary
Frank Lechermann
Summary: Nickelate superconductors of infinite-layer type exhibit challenging electronic properties with doping, leading to rich physics. The superconducting hole-doped region serves as the meeting point of a (self-)doped Mott insulator and a bad Hund metal. The Fermi-level crossing of the Ni-dz(2) flat-band creates a singular arena for unconventional superconductivity.
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Yuan Cao et al.
Summary: The study of magic-angle twisted trilayer graphene has revealed unexpectedly strong superconductivity, surpassing the conventional Pauli limit. The results suggest that external magnetic fields can induce transitions between phases with potentially different order parameters.
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Materials Science, Multidisciplinary
Xiao-Rong Zhou et al.
Summary: The study presents experimental results on a 14-nm-thick superconducting Nd0.8Sr0.2NiO2/SrTiO3 thin-film heterostructure, revealing key performance characteristics such as a relatively small critical current density and complex magnetotransport properties.
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Multidisciplinary Sciences
H. Lu et al.
Summary: The discovery of superconductivity in infinite-layer nickelates brings us closer to a material class similar to cuprate superconductors. Measurements of magnetic excitations in these nickelates showed that undoped NdNiO2 possesses a branch of dispersive excitations with a bandwidth of approximately 200 milli-electron volts.
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F. H. Yu et al.
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NATURE COMMUNICATIONS
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Ying Xiang et al.
Summary: The discovery of superconductivity in infinite-layer nickelate superconducting films has sparked interest due to similarities with high-T(c) cuprate superconductors. Experimental data on these films, specifically regarding the upper critical field, remain limited. This study presents temperature- and angle-dependence of resistivity in Nd0.8Sr0.2NiO2 thin films, revealing information on superconductivity anisotropy and paramagnetic effects.
CHINESE PHYSICS LETTERS
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Nan Zhou et al.
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Peayush Choubey et al.
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Materials Science, Multidisciplinary
Manasi Mandal et al.
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A. S. Botana et al.
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F. Buta et al.
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Xiangang Wan et al.
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