Unveiling the Origin of Co3O4 Quantum Dots for Photocatalytic Overall Water Splitting

Article Chemistry, Multidisciplinary

Enhanced Overall Water Splitting by a Zirconium-Doped TaON-Based Photocatalyst

Jiadong Xiao et al.

Summary: Researchers have synthesized a solar-powered one-step-excitation overall water splitting photocatalyst with improved efficiency by modifying the synthetic precursor and controlling defects.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2022)

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Article Chemistry, Multidisciplinary

Pt Particle Size Affects Both the Charge Separation and Water Reduction Efficiencies of CdS-Pt Nanorod Photocatalysts for Light Driven H-2 Generation

Yawei Liu et al.

Summary: Decreasing the metal catalyst size to nanoclusters or single atoms is a new trend in developing more efficient photocatalytic systems. Research has shown that the size of Pt catalyst has a significant impact on light driven H2 generation efficiency in CdS-Pt heterostructures, with QE(H2) increasing as the Pt size increases.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2022)

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Article Chemistry, Physical

Facet-Oriented Assembly of Mo:BiVO4 and Rh:SrTiO3 Particles: Integration of p-n Conjugated Photo-electrochemical System in a Particle Applied to Photocatalytic Overall Water Splitting

Boyang Zhang et al.

Summary: In this study, a p-n conjugated two-electrode water-splitting system was miniaturized into one particle to achieve photocatalytic water splitting. By visualizing the photoexcited charge migration and accumulation, efficient interfacial charge transfer and effective surface modification were achieved, allowing for visible light-driven overall water splitting.

ACS CATALYSIS (2022)

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Article Chemistry, Multidisciplinary

Atomically Dispersed Janus Nickel Sites on Red Phosphorus for Photocatalytic Overall Water Splitting

Menglong Wang et al.

Summary: Single-atom nickel catalysts prepared on red phosphorus using a reactive-group guided strategy exhibit elevated hydrogen evolution rate under visible-light irradiation due to their specific Janus structure.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2022)

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Article Chemistry, Physical

Heterojunction Design between WSe2 Nanosheets and TiO2 for Efficient Photocatalytic Hydrogen Generation

Xu Guo et al.

Summary: A series of WSe2/TiO2 nanocomposites were constructed through a mechanical grinding method, and all of them exhibited boosted photocatalytic hydrogen evolution. The enhanced performance was attributed to efficient electron transfer and abundant active sites provided by WSe2 nanosheets. The intimate heterojunction between WSe2 nanosheets and TiO2 favored charge separation.

CATALYSTS (2022)

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Article Chemistry, Multidisciplinary

Heterointerface Engineering of ZnO/CdS Heterostructures through ZnS Layers for Photocatalytic Water Splitting

Xu Guo et al.

Summary: Heterostructure catalysts are promising for photocatalytic hydrogen generation, with ZnO/ZnS/CdS and ZnO/CdS heterostructures exhibiting superior performance through heterointerface engineering. These findings contribute significantly to the development of solar-driven water splitting technology.

CHEMISTRY-A EUROPEAN JOURNAL (2022)

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Article Chemistry, Physical

Heteroepitaxial growth of core-shell ZnO/CdS heterostructure for efficient and stable photocatalytic hydrogen generation

Xu Guo et al.

Summary: In this study, colloidal ZnO/CdS heterostructure catalysts were successfully obtained using a two-step heteroepitaxial growth strategy. By optimizing the molar ratio of the ZnO and CdS components, the catalyst exhibited a high hydrogen generation rate and excellent photocatalytic stability. The nanoscale ZnO/CdS heterostructure showed superior photocatalytic performance compared to bulk ZnO/CdS heterostructures.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2022)

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Article Engineering, Environmental

A facile mechanochemical preparation of Co3O4@g-C3N4 for application in supercapacitors and degradation of pollutants in water

Iqra Rabani et al.

Summary: This study successfully synthesized a Co3O4@g-C3N4 hybrid, demonstrating excellent performance in supercapacitor and photocatalyst applications, showing significant pseudocapacitive behavior and high cycling stability.

JOURNAL OF HAZARDOUS MATERIALS (2021)

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Article Physics, Condensed Matter

Co3O4 nanoparticles characterized by XPS and UPS

Kevin M. Cole et al.

Summary: X-ray photoelectron spectroscopy and ultraviolet photoelectron spectroscopy were used to investigate Co3O4 nanoparticles. Detailed analysis of the valence states and surface photoelectron signals of Co3O4 were provided in the study.

SURFACE SCIENCE SPECTRA (2021)

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Article Nanoscience & Nanotechnology

Magnetically Controllable Flowerlike, Polyhedral Ag-Cu-Co3O4 for Surface-Enhanced Raman Scattering

Zheng Fu et al.

Summary: Cu, Ag, and Ag-Cu-Co3O4 nanomaterials with hierarchical flower shapes were synthesized, integrating the optical properties of the core and the magnetic properties of the branches. It was found that Ag-Cu-Co3O4 enhances SERS activity for adsorbed rhodamine 6G, showing potential for tandem SERS detection/magnetic separation applications.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Chemistry, Multidisciplinary

Efficient Photocatalytic Overall Water Splitting Induced by the Giant Internal Electric Field of a g-C3N4/rGO/PDIP Z-Scheme Heterojunction

Xianjie Chen et al.

Summary: The research successfully constructed a graphitic carbon nitride/rGO/perylene diimide polymer (g-C3N4/rGO/PDIP) Z-scheme heterojunction, achieving high-efficiency and stable photocatalytic overall water splitting activity. By building a giant internal electric field in the Z-scheme junction, the charge separation efficiency was significantly improved, leading to higher hydrogen and oxygen evolution rates, quantum efficiency, and solar-to-hydrogen energy conversion efficiency.

ADVANCED MATERIALS (2021)

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Article Chemistry, Physical

Barrierless Self-Trapping of Photocarriers in Co3O4

Yacun Zhang et al.

Summary: The self-trapping of free carriers in transition-metal oxides can lead to small polarons, causing inadequate performance of oxide-based optoelectronic applications. Understanding the self-trapping mechanism is crucial for improving the performance of these applications. The study on Co3O4 epitaxial monocrystalline films using transient absorption spectroscopy revealed a barrierless self-trapping mechanism derived from the small polaron framework.

JOURNAL OF PHYSICAL CHEMISTRY LETTERS (2021)

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Article Chemistry, Multidisciplinary

Slow Auger Recombination of Trapped Excitons Enables Efficient Multiple Electron Transfer in CdS-Pt Nanorod Heterostructures

Yawei Liu et al.

Summary: The study explores the dynamics of multiple electron transfer in CdS-Pt nanorods, revealing the efficiency and competition in multiexciton dissociation and electron transfer processes. This has implications for driving multielectron photocatalytic reactions and controlling product selectivity under intense illumination.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2021)

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Article Chemistry, Multidisciplinary

Selective Cocatalyst Deposition on ZnTiO3-xNy Hollow Nanospheres with Efficient Charge Separation for Solar-Driven Overall Water Splitting

Shunhang Wei et al.

Summary: Pt and RhOx cocatalysts are selectively deposited at inner and outer surface of ZnTiO3-xNy hollow nanospheres, improving photocatalytic overall water splitting activity by promoting efficient dissociation and fast migration of photocarriers.

SMALL (2021)

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Article Chemistry, Multidisciplinary

The Hole-Tunneling Heterojunction of Hematite-Based Photoanodes Accelerates Photosynthetic Reaction

Hongwen Zhang et al.

Summary: The study successfully designed single-atom metal-insulator-semiconductor heterojunctions for efficient CO2 conversion by combining an Al2O3 overlayer with a RuOx hole-collector. The dielectric field played a key role in the charge dynamics at the Al2O3/SF nanorods interface, accelerating the O-2-evolving reaction kinetics. Integration of double SIMS-3 photoanodes with a single-atom Ni-doped graphene CO2-reduction-catalyst cathode achieved high CO-evolution rate and overall quantum efficiency.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Nanoscience & Nanotechnology

Acid-Etched Co3O4 Nanoparticles on Nickel Foam: The Highly Reactive (311) Facet and Enriched Defects for Boosting Methanol Oxidation Electrocatalysis

Yanming Cao et al.

Summary: This study synthesized Co3O4 nanoparticles with superior MOR activity by utilizing an acid etching method and defect construction, mainly due to the exposed (311) facet and abundant oxygen vacancies (V-O) as active sites, as well as the reduced adsorption energy of methanol molecules from phase purification.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Nanoscience & Nanotechnology

Tailored Co3O4-Based Nanosystems: Toward Photocatalysts for Air Purification

Javier Fragoso et al.

Summary: This study focuses on supported Co3O4-based nanomaterials fabricated via chemical vapor deposition, evaluated for the first time as photocatalysts for NO oxidation under sunlight. Heterostructure formation through deposition of SnO2 or Fe2O3 onto Co3O4 was explored, showing a direct dependence of system behavior on the chemical composition, overlayer morphology, and charge transfer events. The results provide valuable guidelines for the future development of improved photocatalysts for air purification.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Chemistry, Multidisciplinary

Two-Dimensional All-in-One Sulfide Monolayers Driving Photocatalytic Overall Water Splitting

Rongrong Pan et al.

Summary: This study demonstrates that ZnIn2S4 monolayers with dual defects show optimized light absorption and carrier dynamics, with the dual defects serving as active sites for water oxidation (Ag dopants) and reduction (nanoholes) to achieve steady performance in photocatalytic overall water splitting without the need for cocatalysts.

NANO LETTERS (2021)

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Article Chemistry, Physical

Investigation into the Enhanced Catalytic Oxidation of o-Xylene over MOF-Derived Co3O4 with Different Shapes: The Role of Surface Twofold-Coordinate Lattice Oxygen (O2f)

Ying Ma et al.

Summary: Co3O4 catalysts with different shapes derived from metal-organic frameworks exhibit enhanced catalytic oxidation of o-xylene, with the active surface oxygen species O-2f playing a crucial role in oxygen vacancy formation and gaseous oxygen replenishment, leading to improved catalytic performance.

ACS CATALYSIS (2021)

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Article Chemistry, Multidisciplinary

Accelerating the oxygen evolution reaction kinetics of Co3O4 in neutral electrolyte by decorating RuO2

Kaifa Lu et al.

Summary: Efficient electrocatalysts for the neutral oxygen evolution reaction are crucial yet challenging. Through a combination of density functional theory calculations and experiments, it has been demonstrated that the decoration of RuO2 can greatly enhance the OER kinetics of Co3O4 in neutral electrolyte. RuO2-decorated Co3O4 shows high activity (365 mV at 10 mA cm(-2)) and decent stability (up to 100 hours) in 1 M PBS electrolyte.

CHEMICAL COMMUNICATIONS (2021)

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Article Chemistry, Physical

Unravelling intramolecular charge transfer in donor-acceptor structured g-C3N4 for superior photocatalytic hydrogen evolution

Chenglu Zhu et al.

Summary: The incorporation of 2-aminobenzothiazole (ABT) into the g-C3N4 framework led to the synthesis of a series of D-A structured photocatalysts with improved performance. The enhanced photocatalytic hydrogen evolution was attributed to the broadened visible light absorption range and accelerated charge carrier separation due to ultrafast intramolecular charge transfer. The boosted performance is closely related to the deliberately introduced D-A structure, which may offer insights for designing analogues with better photocatalytic hydrogen evolution performance.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Article Chemistry, Physical

Highly efficient photocatalytic water splitting utilizing a WO3-x/ZnIn2S4 ultrathin nanosheet Z-scheme catalyst

Dian Luo et al.

Summary: A highly crimped WO3-x/ZnIn2S4 flexible ultrathin nanosheet heterojunction was synthesized for enhanced photocatalytic hydrogen evolution. The heterojunction exhibited highly efficient hydrogen production activity with an apparent quantum efficiency of 26.28% at 400 nm.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Article Engineering, Environmental

Few-layer WSe2 nanosheets as an efficient cocatalyst for improved photocatalytic hydrogen evolution over Zn0.1Cd0.9S nanorods

Xu Guo et al.

CHEMICAL ENGINEERING JOURNAL (2020)

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Article Green & Sustainable Science & Technology

Co3O4 imbedded g-C3N4 heterojunction photocatalysts for visible-light-driven hydrogen evolution

Lingyan Yang et al.

RENEWABLE ENERGY (2020)

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Article Chemistry, Physical

Yolk-shell-like mesoporous CoCrOx with superior activity and chlorine resistance in dichloromethane destruction

Xiangbo Feng et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2020)

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Article Chemistry, Multidisciplinary

Engineering of Electronic States on Co3O4 Ultrathin Nanosheets by Cation Substitution and Anion Vacancies for Oxygen Evolution Reaction

Qichen Wang et al.

SMALL (2020)

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Article Chemistry, Multidisciplinary

Enhanced Photocatalytic H2-Production Activity of CdS Quantum Dots Using Sn2+ as Cocatalyst under Visible Light Irradiation

Xianglin Xiang et al.

SMALL (2020)

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Review Chemistry, Multidisciplinary

Recent Advances in Conjugated Polymers for Visible-Light-Driven Water Splitting

Chengxiao Zhao et al.

ADVANCED MATERIALS (2020)

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Article Nanoscience & Nanotechnology

Enhanced Light-Driven Charge Separation and H2 Generation Efficiency in WSe2 Nanosheet-Semiconductor Nanocrystal Heterostructures

Xu Guo et al.

ACS APPLIED MATERIALS & INTERFACES (2020)

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Article Nanoscience & Nanotechnology

Co3O4 Nanocrystals with an Oxygen Vacancy-Rich and Highly Reactive (222) Facet on Carbon Nitride Scaffolds for Efficient Photocatalytic Oxygen Evolution

Yunxiong Zeng et al.

ACS APPLIED MATERIALS & INTERFACES (2020)

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Article Chemistry, Physical

Beyond Hydrogen Evolution: Solar-Driven, Water-Donating Transfer Hydrogenation over Platinum/Carbon Nitride

Chenhui Han et al.

ACS CATALYSIS (2020)

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Article Chemistry, Physical

Insights into High-Performance Monolith Catalysts of Co3O4 Nanowires Grown on Nickel Foam with Abundant Oxygen Vacancies for Formaldehyde Oxidation

Kaiwen Zha et al.

ACS CATALYSIS (2020)

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Article Chemistry, Multidisciplinary

Unraveling the Interfacial Charge Migration Pathway at the Atomic Level in a Highly Efficient Z-Scheme Photocatalyst

Pengfei Wang et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2019)

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Atomic-Scale Insights into the Low-Temperature Oxidation of Methanol over a Single-Atom Pt1-Co3O4 Catalyst

Zeyu Jiang et al.

ADVANCED FUNCTIONAL MATERIALS (2019)

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Charge Separation, Band-Bending, and Recombination in WO3 Photoanodes

Sacha Corby et al.

JOURNAL OF PHYSICAL CHEMISTRY LETTERS (2019)

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Roles of Charge Carriers in the Excited State Dynamics of BiVO4 Photoanodes

Abdullah Kahraman et al.

JOURNAL OF PHYSICAL CHEMISTRY C (2019)

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Rational design of CrOx/LaSrMnCoO6 composite catalysts with superior chlorine tolerance and stability for 1,2-dichloroethane deep destruction

Mingjiao Tian et al.

APPLIED CATALYSIS A-GENERAL (2019)

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Insight into the boosted catalytic performance and chlorine resistance of nanosphere-like meso-macroporous CrOx/MnCo3Ox for 1,2-dichloroethane destruction

Mingjiao Tian et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2019)

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Ultrafast Charge Separation in Two-Dimensional CsPbBr3 Perovskite Nanoplatelets

Quyang Li et al.

JOURNAL OF PHYSICAL CHEMISTRY LETTERS (2019)

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ZnO nanorods modified with noble metal-free Co3O4 nanoparticles as a photocatalyst for efficient ethylene degradation under light irradiation

Zihao Cui et al.

CATALYSIS SCIENCE & TECHNOLOGY (2019)

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Noble metal-free integrated UiO-66-PANI-Co3O4 catalyst for visible-light-induced H2 production

Ajay K. Singh et al.

CHEMICAL COMMUNICATIONS (2019)

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The chemically reduced CuO-Co3O4 composite as a highly efficient electrocatalyst for oxygen evolution reaction in alkaline media

Umair Aftab et al.

CATALYSIS SCIENCE & TECHNOLOGY (2019)

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g-C3N4/CuO and g-C3N4/Co3O4 nanohybrid structures as efficient electrode materials in symmetric supercapacitors

Jithesh Kavil et al.

RSC ADVANCES (2019)

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ACS CATALYSIS (2018)

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Size-Dependent Band-Gap and Molar Absorption Coefficients of Colloidal CuInS2 Quantum Dots

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Two-Dimensional Morphology Enhances Light-Driven H-2 Generation Efficiency in CdS Nanoplatelet-Pt Heterostructures

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JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2018)

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Catalytic removal of 1,2-dichloroethane over LaSrMnCoO6/H-ZSM-5 composite: insights into synergistic effect and pollutant-destruction mechanism

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Water Oxidation and Electron Extraction Kinetics in Nanostructured Tungsten Trioxide Photoanodes

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JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2018)

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Facet-Selective Growth of Cadmium Sulfide Nanorods on Zinc Oxide Microrods: Intergrowth Effect for Improved Photocatalytic Performance

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CHEMCATCHEM (2018)

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Co3O4-δ Quantum Dots As a Highly Efficient Oxygen Evolution Reaction Catalyst for Water Splitting

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One-step hydrothermal synthesis of ZnxCdi1-xS/ZnO heterostructures for efficient photocatalytic hydrogen production

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INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2016)

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Putting DFT to the Test: A First-Principles Study of Electronic, Magnetic, and Optical Properties of Co3O4

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Co3O4 quantum dots: reverse micelle synthesis and visible-light-driven photocatalytic overall water splitting

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Long-Lived Photoexcited Carrier Dynamics of d-d Excitations in Spinel Ordered Co3O4

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Characterization of Photo-Induced Charge Transfer and Hot Carrier Relaxation Pathways in Spinel Cobalt Oxide (Co3O4)

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Hole Removal Rate Limits Photodriven H2 Generation Efficiency in CdS-Pt and CdSe/CdS-Pt Semiconductor Nanorod-Metal Tip Heterostructures

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Charge Carrier Dynamics of Photoexcited Co3O4 in Methanol: Extending High Harmonic Transient Absorption Spectroscopy to Liquid Environments

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Visible Light Induced Hole Transport from Sensitizer to Co3O4 Water Oxidation Catalyst across Nanoscale Silica Barrier with Embedded Molecular Wires

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In situ probe of photocarrier dynamics in water-splitting hematite (α-Fe2O3) electrodes

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Resolving surface chemical states in XPS analysis of first row transition metals, oxides and hydroxides: Cr, Mn, Fe, Co and Ni

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F-Doped Co3O4 Photocatalysts for Sustainable H2 Generation from Water/Ethanol

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Solubility-controlled synthesis of high-quality Co3O4 nanocrystals

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GaN:ZnO solid solution as a photocatalyst for visible-light-driven overall water splitting

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Unveiling the Origin of Co3O4 Quantum Dots for Photocatalytic Overall Water Splitting

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