4.6 Article

Investigation of the thermoluminescence dosimeter characteristics of multilayer ZnO(300 nm)/Ag(50 nm)/ZnO(x) thin films for photonic dosimetry applications

Journal

OPTICAL MATERIALS
Volume 137, Issue -, Pages -

Publisher

ELSEVIER
DOI: 10.1016/j.optmat.2023.113548

Keywords

Dosimetry; Ag-ZnO; Thermoluminescence; Radiation; Photonic dosimetry; TLD

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This study introduces a new sensor for photonic dosimetry, synthesized using RF sputtering at 300 degrees C. The dosimetric properties were investigated for X-ray doses up to 4 Gy, showing a linear dose-response. The system ZnO(300 nm)/Ag(50 nm)/ZnO(x nm) exhibited the highest thermoluminescence intensity and a single peak in the glow curve at 246 degrees C. Various dosimeter parameters, such as homogeneity, precision, and fading properties, were examined, and the proposed dosimeter showed good radiation-measuring characteristics.
This study demonstrated a novel sensor based on a semiconductor-metal-semiconductor multilayer film for photonic dosimetry that was synthesized at 300 degrees C using radiofrequency RF sputtering. The dosimetric properties of samples exposed to X-ray doses of up to 4 Gy were investigated. The system ZnO(300 nm)/Ag(50 nm)/ZnO(x nm) was chosen based hiest thermoluminescence TL intensity. The glow curve exhibited a single peak with a maximum temperature peak Tm of 246 degrees C. In addition, the proposed dosimeter has a linear dose-response up to 4 Gy. The heating rate with the highest TL intensity was 3 degrees C/s. The best annealing protocol for optimal TL intensity and minimum standard deviation was found at 200 degrees C and 30 min. Most dosimeter parameters were investigated, including homogeneity, precision, and fading properties. . The kinetic parameters of the dosimeter were calculated and employed two methods: peak shape and initial rise. The results showed that the trap has activation energies at 0.51 and 0.53 eV and frequency factor between 0.25 x 108 and 0.5 x 109. Other features, like recycling, the receding of TL at room temperature, and optical fading, have been investigated. The suggested dosimeter demonstrated good radiation-measuring characteristics. The glow curve was immediately acquired, the annealing process was uncomplicated, and the dosimeter had a high sensitivity of 1.49 of TLD-100, making it suitable for radiation monitoring.

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