4.8 Article

Synthesis of an all-carbon conjugated polymeric segment of carbon nanotubes and its application for lithium-ion batteries

Journal

NANO RESEARCH
Volume -, Issue -, Pages -

Publisher

TSINGHUA UNIV PRESS
DOI: 10.1007/s12274-023-5530-4

Keywords

carbon nanomaterials; conjugated polymer; carbon nanotubes; lithium-ion batteries

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In this paper, the design and synthesis of a novel all-carbon conjugated polymeric segment of single-walled carbon nanotubes (poly(cyclo-para-phenylene) (PCPP)) and its first application as an anode material for lithium-ion batteries were reported. The as-synthesized PCPP was characterized by Raman spectroscopy, Fourier transform infrared (FTIR), and other spectroscopies. The electrochemical characterization results showed the suitability of PCPP as an anode material for lithium-ion batteries. Theoretical calculations indicated the unique structural and physical properties of PCPP. The realization of PCPP expanded the scope of bottom-up synthesis of uniform carbon nanotube segments and their potential applications as new materials for lithium-ion batteries.
The synthesis and potential applications of nanocarbon materials have attracted much attention in recent years. Herein, we report the design and synthesis of a novel all-carbon conjugated polymeric segment of single-walled carbon nanotubes (poly(cyclo-para-phenylene) (PCPP)) and its first application as an anode material for lithium-ion batteries. The as-synthesized PCPP was characterized by Raman spectroscopy, Fourier transform infrared (FTIR), and other spectroscopies. The electrochemical characterization results show the suitability of PCPP as an anode material for lithium-ion batteries. Theoretical calculations indicate the unique structural and physical properties of PCPP. The realization of PCPP expands the scope of bottom-up synthesis of uniform carbon nanotube segments and their potential applications as new materials for lithium-ion batteries.

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