Journal
MATERIALS LETTERS
Volume 339, Issue -, Pages -Publisher
ELSEVIER
DOI: 10.1016/j.matlet.2023.134099
Keywords
Pyrazine; One-dimensional perovskite; Structure; Efficiency; Solar cells
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The synthesis, crystal structures, optical band gaps, and device applications of (C4N2H6)PbI3 and (C4N2H6)PbBr3 were investigated and discussed. 1D perovskite single crystals based on pyrazine were successfully obtained by reacting the organic cation C4N2H6 with lead iodide and bromide. The compounds (C4N2H6)PbI3 and (C4N2H6)PbBr3 have band gaps of 2.71 and 2.82 eV, respectively, which are consistent with their structural distortion. The 1D crystals of (Py)PbI3 and (Py)PbBr3 contributed to the enhancement of device efficiency to 22.12% and 22.38%, respectively.
Here, the crystal synthesis, crystal structures, optical band gaps and application in devices of (C4N2H6)PbI3 and (C4N2H6)PbBr3 are researched and discussed. Novel hybrid 1D perovskite single crystals based on pyrazine were obtained by reacting the organic cation C4N2H6 with lead iodide and bromide. The band gaps of (C4N2H6)PbI3 and (C4N2H6)PbBr3 compounds are 2.71 and 2.82 eV, respectively, which consistent with the structure distor-tion. The 1D crystals of (Py)PbI3 and (Py)PbBr3 assisted the device efficiency from 20.15% to 22.12 and 22.38%, respectively.
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