Journal
ADVANCED MATERIALS
Volume 27, Issue 39, Pages 6046-6054Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adma.201503218
Keywords
2D-conjugated polymers; anisotropy; interfaces; molecular orientation; polymer solar cells
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Funding
- National Basic Research Program 973 [2014CB643501]
- NSFC [91333204, 51261160496]
- Chinese Academy of Sciences [XDB12030200]
- US Department of Energy, Office of Science, Basic Energy Science, Division of Materials Science and Engineering [DE-FG02-98ER45737]
- Office of Science, Office of Basic Energy Sciences, of the US Department of Energy [DE-AC02-05CH11231]
- CAS-Croucher Funding Scheme for Joint Labs
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Manipulating molecular orientation at the donor/acceptor interface is the key to boosting charge separation properties and efficiencies of anisotropic-materials-based organic photovoltaics (OPVs). By replacing the polymeric donor PBDTBDD with its 2D-conjugated polymer PBDTBDD-T, the power conversion efficiency of OPVs featuring the anisotropic polymer acceptor PNDI is drastically boosted from 2.4% up to 5.8%.
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