Journal
ADVANCED MATERIALS
Volume 27, Issue 39, Pages 5989-5994Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adma.201502024
Keywords
calcium-manganese oxides; e(g) electron filling; electronic state transitions; oxygen evolution reactions; spin behaviors
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Funding
- National Basic Research Program of China [2015CB932302]
- National Natural Science Foundation of China [21222101, U1432133, 11132009, 21331005, 11321503, J1030412]
- Chinese Academy of Sciences [XDB01020300]
- Fok Ying-Tong Education Foundation, China [141042]
- Fundamental Research Funds for the Central Universities [WK2060190027, WK2060190031]
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A surface hydrogen effect to modulate the pure electronic-state transition in perovskite Ca0.9Yb0.1MnO3 synergistically generates a more suitable e(g) electron filling status and better conductivity. This achieves 100 times higher catalytic activity compared to that of a pristine sample.
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