Journal
JOURNAL OF THE BRAZILIAN CHEMICAL SOCIETY
Volume 27, Issue 11, Pages 2034-2045Publisher
SOC BRASILEIRA QUIMICA
DOI: 10.5935/0103-5053.20160093
Keywords
zeolite; coal fly ash; toxic element; element distribution
Categories
Funding
- CNPq
- FAPERGS/CAPES
- FAPERGS
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Coal fly ash has been proposed as an alternative raw material for zeolite synthesis, however, the mobilization of toxic elements of this material into zeolite products, washing water and effluent is rarely addressed. In this study, Brazilian coal fly ash was used in the integrated synthesis (two steps) of zeolites Na-P1 and 4A and the distribution of approximately 40 major, minor and trace elements was investigated in all the input and output flows involved in the process. The mobilization of several elements was observed in the zeolite products, a number of which are highly toxic, such as As, Cd, Cr, Ni and Pb. With regard to the amount present in the ash, both zeolites were enriched in several elements, such as Ni in zeolite Na-P1 and As in zeolite 4A. The latter exhibited high purity, with most of the elements investigated having concentrations close to those measured in commercial zeolite 4A. Important information was gathered regarding zeolite synthesis using fly ash, which will ensure safer application of these materials and, if necessary, propose a contaminant-free synthesis route.
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