Journal
CHEMPHYSCHEM
Volume 24, Issue 12, Pages -Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cphc.202300001
Keywords
electronic coherence; femtochemistry; fluorescence; lanthanides; wave packets
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Temporally delayed, phase-locked coherent pairs of near IR femtosecond laser pulses were used to investigate electronic coherences in molecular Nd3+-complexes at room temperature. Dissolved and solid complexes were studied using a confocal microscope with fluorescence detection. The observed electronic coherence on a few hundred femtoseconds time scale is modulated by additional coherent wave packet dynamics, mainly attributed to vibrations. In the future, these complexes could serve as prototypes for potential applications in quantum information technology.
Temporally delayed, phase-locked coherent pairs of near IR femtosecond laser pulses were employed to study electronic coherences in molecular Nd3+-complexes at room temperature. Dissolved and solid complexes were studied under a confocal microscope set-up with fluorescence detection. The observed electronic coherence on a few hundred femtoseconds time scale is modulated by additional coherent wave packet dynamics, which we attribute mainly to be vibrational in nature. In future, the complexes may serve as prototypes for possible applications in quantum information technology.
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