4.7 Article

Superhydrophobic, stretchable kirigami pencil-on-paper multifunctional device platform

Journal

CHEMICAL ENGINEERING JOURNAL
Volume 465, Issue -, Pages -

Publisher

ELSEVIER SCIENCE SA
DOI: 10.1016/j.cej.2023.142774

Keywords

Superhydrophobic; Pencil-on-paper; Multiparameter sensing; Thermal therapy and electrical stimulation; Personal and population health monitoring

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This paper introduces a new type of wearable electronic device that combines pencil-on-paper with a hydrophobic coating and stretchable kirigami structures to create a superhydrophobic and stretchable multifunctional sensing platform. The resulting sensor exhibits a large response to NO2 gas and is minimally affected by variations in temperature, humidity, and mechanical deformations. It can be used to detect temperature and electrophysiological signals and provide thermal therapy and electrical stimulation for various medical applications.
Wearable electronics with applications in healthcare, human-machine interfaces, and robotics often explore complex manufacturing procedures and are not disposable. Although the use of conductive pencil patterns on cellulose paper provides inexpensive, disposable sensors, they have limited stretchability and are easily affected by variations in the ambient environment. This work presents the combination of pencil-on-paper with the hydrophobic fumed SiO2 (Hf-SiO2) coating and stretchable kirigami structures from laser cutting to prepare a superhydrophobic, stretchable pencil-on-paper multifunctional sensing platform. The resulting sensor exhibits a large response to NO2 gas at elevated temperature from self-heating, which is minimally affected by the variations in the ambient temperature and relative humidity, as well as mechanical deformations such as bending and stretching states. The integrated temperature sensor and electrodes with the sensing platform can accurately detect temperature and electrophysiological signals to alert for adverse thermal effects and cardiopulmonary diseases. The thermal therapy and electrical stimulation provided by the platform can also deliver effective means to battle against inflammation/infection and treat chronic wounds. The superhydrophobic pencil-onpaper multifunctional device platform provides a low-cost, disposable solution to disease diagnostic confirmation and early treatment for personal and population health.

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