Journal
APPLIED PHYSICS LETTERS
Volume 122, Issue 13, Pages -Publisher
AIP Publishing
DOI: 10.1063/5.0146081
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Two-dimensional multiferroic materials are explored through structural design and molecular engineering for robust magnetoelectric coupling and controllable topological solitons. This review focuses on the design of multiferroic structures in the 2D form, achieving robust magnetoelectric coupling, and electrically controlling magnetic skyrmions via multiferroic effects. Challenges and opportunities for predicting 2D multiferroic materials are discussed.
Two-dimensional (2D) multiferroic materials with robust magnetoelectric coupling and controllable topological solitons (such as skyrmions) are promising candidates for advanced information storage and processing. Due to the limitations of experimental techniques, first-principles investigations stand out in answering fundamental questions of 2D multiferroic couplings, thus providing guidance for experimental validation. Herein, we will give a review of recent theoretical progress in the exploration of 2D multiferroic coupling via structural design and molecular engineering approach. Particularly, we will focus on (i) how to design the multiferroic structure in the 2D form; (ii) how to achieve robust magnetoelectric coupling; and (iii) how to electrically control the magnetic skyrmion via multiferroic effects. Finally, we give some perspectives on the remaining challenges and opportunities for predicting 2D multiferroic materials.
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