Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 138, Issue 32, Pages 10080-10083Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jacs.6b05498
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Funding
- Ministry of Science and Technology of China [2013CB834505, 2013CB834804, 2014CB239402]
- National Natural Science Foundation of China [21390404, 91427303, 21402217]
- Chinese Academy of Sciences
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We present a blueprint for aromatic C-H functionalization via a combination of photocatalysis and cobalt catalysis and describe the utility of this strategy for benzene amination and hydroxylation. Without any sacrificial oxidant, we could use the dual catalyst systeth to produce aniline directly from benzene and ammonia, and phenol from benzene and water, both with evolution of hydrogen gas under unusually mild conditions in excellent yields and selectivities.
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