Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 138, Issue 38, Pages 12308-12311Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jacs.6b05865
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Funding
- French National Research Agency [ANR-11-LABX-0003-01]
- European Research Council under the European Union/ERC [306398]
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Dye-sensitized photoelectrochemical cells (DS-PECs) for water splitting hold promise for the large-scale storage of solar energy in the form of (solar) fuels, owing to the low cost and ease to process of their constitutive photoelectrode materials. The efficiency of such systems ultimately depends on our capacity to promote unidirectional light-driven electron transfer from the electrode substrate to a catalytic moiety. We report here on the first noble-metal free and covalent dye-catalyst assembly able to achieve photoelectrochemical visible light-driven H-2 evolution in mildly acidic aqueous conditions when grafted onto p-type NiO electrode substrate
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