Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 138, Issue 32, Pages 10088-10091Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jacs.6b05552
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Funding
- JST, CREST program
- Ministry of Education, Culture, Sports, Science and Technology, Government of Japan [2401]
- Grants-in-Aid for Scientific Research [16H06508, 15H00735, 16H06517, 16J11419] Funding Source: KAKEN
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A series of conductive porous composites were obtained by the polymerization of 3,4-ethylenedioxythiophene (EDOT) in the cavities of MIL-101(Ci). By controlling the amount of EDOT loaded into the host framework, it was possible to modulate the conductivity as well as the porosity of the composite. This approach yields materials with a reasonable electronic conductivity (1.1 X 10(-3) S.cm(-1)) while maintaining high porosity (S-BET = 803 m(2)/g). This serves as a promising strategy for obtaining highly nanotextuted conductive polymers with very high accessibility for small gas molecules, which are beneficial to the fabrication of a chemiresistive sensor for the detection of NO2.
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